Innovative rapid synthesis design of water-stable solid-state Cs4PbBr6 perovskite luminescence materials for next generation display technology
Source abstract
Abstract
Abstract We demonstrate for the first time a rapid large-scale procedure using planetary centrifugal mixer equipment for the synthesis of green-emitting solid-state Cs4PbBr6 perovskite luminescence materials to improve the efficiency of the synthesis reaction. Compared with the conventional stirring method, the Cs4PbBr6 perovskite materials synthesized with our proposed method display a high photoluminescence quantum yield of 34%. In addition, the surface of the solid-state Cs4PbBr6 luminescence material was modified with a silane coupling agent by the plasma-assisted method. The stability in moisture was improved by the hydrophobic properties imparted to the surface of the Cs4PbBr6. Consequently, in accelerated aging testing, the surface-modified Cs4PbBr6 showed a 20% improvement in the degradation of the photoluminescence property against moisture over that of its counterpart.
Source: openaire · Quality: candidate unverified · Source record ↗
Research context
OpenAlex topics: Perovskite Materials and Applications · Solid-state spectroscopy and crystallography · Luminescence Properties of Advanced Materials
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References (34)
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1. Metal halide perovskite nanomaterials: synthesis and applications10.1039/C6SC04474C ↗
2. Halide perovskites for applications beyond photovoltaics10.1002/smtd.201700310 ↗
3. Perovskite photonic sources10.1038/nphoton.2016.62 ↗
4. Bright light-emitting diodes based on organometal halide perovskite10.1038/nnano.2014.149 ↗
5. Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors10.1038/nmat4271 ↗
6. Park · 2016
7. Thin film perovskite light-emitting diode based on CsPbBr 3 powders and interfacial engineering10.1016/j.nanoen.2017.05.005 ↗
8. All-inorganic colloidal perovskite quantum dots: a new class of lasing materials with favorable characteristics10.1002/adma.201503573 ↗
9. High-efficiency light-emitting diodes of organometal halide perovskite amorphous nanoparticles10.1021/acsnano.6b01540 ↗
10. Photoresponse of CsPbBr 3 and Cs4PbBr6 perovskite single crystals10.1021/acs.jpclett.6b02763 ↗
11. Organometal halide perovskites as visible-light sensitizers for photovoltaic cells10.1021/ja809598r ↗
12. 6.5% efficient perovskite quantum-dot-sensitized solar cell10.1039/c1nr10867k ↗
13. Methodologies toward highly efficient perovskite solar cells10.1002/smll.201704177 ↗
14. An interface stabilized perovskite solar cell with high stabilized efficiency and low voltage loss10.1039/C9EE00751B ↗
15. Ligand mediated transformation of cesium lead bromide perovskite nanocrystals to lead depleted Cs4PbBr 6 nanocrystals10.1021/jacs.7b01409 ↗
16. Pure Cs4PbBr 6: highly luminescent zero-dimensional perovskite solids10.1021/acsenergylett.6b00396 ↗
17. Intrinsic lead ion emissions in zero-dimensional Cs4PbBr 6 nanocrystals10.1021/acsenergylett.7b01026 ↗
18. Solution-grown CsPbBr 3/Cs4PbBr6 perovskite nanocomposites: toward temperature-insensitive optical gain
19. Zero-dimensional Cs4PbBr 6 perovskite nanocrystals10.1021/acs.jpclett.7b00105 ↗
20. Continuous synthesis of highly stable Cs4PbBr 6 perovskite microcrystals by a microfluidic system and their application in white-light-emitting diodes10.1021/acs.inorgchem.8b01985 ↗
21. Non-injection gram-scale synthesis of cesium lead halide perovskite quantum dots with controllable size and composition10.1007/s12274-016-1090-1 ↗
22. Ten-gram-scale synthesis of FAPbX3 perovskite nanocrystals by a high-power room-temperature ultrasonic-assisted strategy and their electroluminescence10.1002/admt.201901089 ↗
23. Room-temperature and gram-scale synthesis of CsPbX3 (X = Cl, Br, I) perovskite nanocrystals with 50–85% photoluminescence quantum yields10.1039/C6CC01500J ↗
24. Innovatively continuous mass production couette-taylor flow: pure inorganic green-emitting Cs4PbBr 6 perovskite microcrystal for display technology10.1038/s41598-018-20376-3 ↗
25. Improving the Stability of Metal Halide Perovskite Materials and Light-Emitting Diodes10.1002/adma.201704587 ↗
26. Highly luminescent and ultrastable CsPbBr 3 perovskite quantum dots incorporated into a silica/alumina monolith10.1002/anie.201703264 ↗
27. Design of long-term stable red-emitting CsPb(Br 0.4, I0.6)3 perovskite quantum dot film for generation of warm white light10.1016/j.cej.2016.12.087 ↗
28. Mesoporous silica particles integrated with all-inorganic CsPbBr 3 perovskite quantum-dot nanocomposites (MP-PQDs) with high stability and wide color gamut used for backlight display10.1002/anie.201603698 ↗
29. Ultrastable, highly luminescent organic-inorganic perovskite-polymer composite films10.1002/adma.201603964 ↗
30. Super-hydrophobic cesium lead halide perovskite quantum dot-polymer composites with high stability and luminescent efficiency for wide color gamut white light-emitting diodes10.1021/acs.chemmater.8b04596 ↗
31. In situ crystallization synthesis of CsPbBr 3 perovskite quantum dot-embedded glasses with improved stability for solid-state lighting and random upconverted lasing10.1021/acsami.8b05155 ↗
32. Controlling surface property of K2SiF6:Mn4+ for improvement of lighting-emitting diode reliability10.1016/j.jpcs.2018.01.020 ↗
33. Effects of soybean oil modified cellulose fibril and organosilane modified cellulose fibril on crystallization of polypropylene10.1155/2015/741242 ↗
34. All-inorganic perovskite nanocrystals with a stellar set of stabilities and their use in white light-emitting diodes10.1021/acsami.8b13553 ↗