journal article·2019-04-01Open access

Plasmon-exciton coupling in nanostructured metal-semiconductor composite films

Viktoriia V. Savchuk, Roman V. Gamernyk, Ihor S. Virt, Serhiy Z. Malynych, Anatoliy O. Pinchuk

AIP Advances· Volume 9· Issue 4

Abstract

Nonlinear optical response of metal-semiconductor Zn0.8Co0.2O/Au nanocomposite films was studied experimentally and theoretically. Z-scan measurements revealed a positive nonlinear index of refraction of the composite film. Fluorescent spectroscopy measurements exhibited a narrow sharp peak that might be attributed to exciton peak of semiconductor nanostructured thin film enhanced by nearby gold nanoparticles. Classical electrodynamic calculations of a quantum dot in close proximity to a gold nanoparticle agree well with the experimentally observed normalized quantum efficiency.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Gold and Silver Nanoparticles Synthesis and Applications · Quantum Dots Synthesis And Properties · Plasmonic and Surface Plasmon Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics and Energy Sciences, University of Colorado Colorado Springs, and Center for Biofrontiers Institute, University of Colorado 1 , 1420 Austin Bluffs Parkway 80918, Colorado Springs, Colorado, USA

Department of Physics, Ivan Franko National University of Lviv 2 , 79005 Lviv, Ukraine

Department of Engineering Science and Technology, Ivan Franko Drogobych State Pedagogical University 3 , 82106 Drogobych, Ukraine

Department of Electromechanics and Electronics, Hetman Petro Sahaidachnyi National Army Academy 4 , 79012 Lviv, Ukraine

Department of Photonics, Lviv Polytechnic National University 5 , 79013 Lviv, Ukraine

Funding

Ministry of Education and Science of Ukraine · BioFrontiers Institute, University of Colorado Colorado Springs

References (22)

Show source-provided references
1. Emission quenching of magnetic dipole transitions near a metal nanoparticle10.1021/acsphotonics.5b00397 ↗
2. Exciton-plasmon interactions in metal-semiconductor nanostructures10.1021/jz101102e ↗
3. Plexcitonic quenching by resonant electron transfer from quantum emitter to metallic nanoantenna10.1021/nl403160s ↗
4. Exciton-plasmon interaction and hybrid excitons in semiconductor-metal nanoparticle assemblies10.1021/nl0602140 ↗
5. Optical excitations of hybrid metal-semiconductot nanoparticles
6. Exciton-plasmon couplings in plexcitonic CuCl-Ag nanoshells: Rabi splitting and induced transparency10.1364/josab.31.002273 ↗
7. Observation of selective plasmon-exciton coupling in nonradiative energy transfer: Donor-selective versus acceptor-selective10.1021/nl4009106 ↗
8. 2012
9. Surface-enhanced emission from single semiconductor nanocrystals
10. Enhancement and quenching of single-Molecule Fluorescence
11. Radiative and nonradiative rates of phosphors attached to gold nanoparticles10.1021/nl070623b ↗
12. Enhancement of single-molecule fluorescence using a gold nanoparticle as an optical nanoantenna10.1103/physrevlett.97.017402 ↗
13. Recent advances in ZnO-based light-emitting diodes10.1109/ted.2009.2033769 ↗
14. Surface engineering of ZnO thin film for high efficiency planar perovskite solar cells
15. High-performance ZNO thin-film transistor fabricated by atomic layer deposition
16. Well-defined Au/ZnO nanoparticle composites exhibiting enhanced photocatalytic activities10.1021/am201221x ↗
17. Exciton-plasmon interaction and nonlinear-optical properties of Zn0.8Co0.2O/Au nanoparticles composite film
18. Structure optical properties and synthesis of Co-doped ZnO superstructures10.1007/s13204-012-0077-9 ↗
19. The optical properties of metal nanoparticles: The influence of size, shape, and dielectric environment10.1021/jp026731y ↗
20. High sensitivity, single beam n2 measurements10.1364/ol.14.000955 ↗
21. Spatial coherency of light and nonlinear optical properties of colloidal gold studied by CW Z-scan technique10.17756/nwj.2016-021 ↗
22. 1983