journal article·2023-09-01Open access

Can a deep-learning model make fast predictions of vacancy formation in diverse materials?

Kamal Choudhary, Bobby G. Sumpter

AIP Advances· Volume 13· Issue 9

Abstract

The presence of point defects, such as vacancies, plays an important role in materials design. Here, we explore the extrapolative power of a graph neural network (GNN) to predict vacancy formation energies. We show that a model trained only on perfect materials can also be used to predict vacancy formation energies (Evac) of defect structures without the need for additional training data. Such GNN-based predictions are considerably faster than density functional theory (DFT) calculations and show potential as a quick pre-screening tool for defect systems. To test this strategy, we developed a DFT dataset of 530 Evac consisting of 3D elemental solids, alloys, oxides, semiconductors, and 2D monolayer materials. We analyzed and discussed the applicability of such direct and fast predictions. We applied the model to predict 192 494 Evac for 55 723 materials in the JARVIS-DFT database. Our work demonstrates how a GNN-model performs on unseen data.
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Research context

OpenAlex topics: Machine Learning in Materials Science · X-ray Diffraction in Crystallography · Inorganic Chemistry and Materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Materials Science and Engineering Division, National Institute of Standards and Technology 1 , Gaithersburg, Maryland 20899, USA

Center for Nanophase Materials Sciences, Oak Ridge National Laboratory 2 , Oak Ridge, Tennessee 37831, USA

Funding

National Institute of Standards and Technology · Oak Ridge National Laboratory

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