journal article·2021-12Open access

Domain Wall Patterning and Giant Response Functions in Ferrimagnetic Spinels

Lazar L. Kish, Alex Thaler, Minseong Lee, Alexander V. Zakrzewski, Dalmau Reig‐i‐Plessis, Brian A. Wolin, Xu Wang, Kenneth C. Littrell, Raffi Budakian, Haidong Zhou, Zheng Gai, Matthias D. Frontzek, Vivien S. Zapf, Adam A. Aczel, Lisa DeBeer‐Schmitt, Gregory J. MacDougall

Advanced Science· Volume 8· Issue 23

Abstract

Abstract The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential is not yet realized in the field of magnetism. This work shows a direct connection between magnetic response functions in mechanically strained samples of Mn 3 O 4 and MnV 2 O 4 and stripe‐like patternings of the bulk magnetization which appear below known magnetostructural transitions. Building off previous magnetic force microscopy data, a small‐angle neutron scattering is used to show that these patterns represent distinctive magnetic phenomena which extend throughout the bulk of two separate materials, and further are controllable via applied magnetic field and mechanical stress. These results are unambiguously connected to the anomalously large magnetoelastic and magnetodielectric response functions reported for these materials, by performing susceptibility measurements on the same crystals and directly correlating local and macroscopic data.
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Research context

OpenAlex topics: Multiferroics and related materials · Ferroelectric and Piezoelectric Materials · Magnetic and transport properties of perovskites and related materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics and Materials Research Laboratory University of Illinois at Urbana‐Champaign Urbana IL 61801 USA

Neutron Scattering Division Oak Ridge National Laboratory Oak Ridge TN 37831 USA

National High Magnetic Field Laboratory Los Alamos National Laboratory Los Alamos NM 87544 USA

Department of Physics and Astronomy and Quantum Matter Institute University of British Columbia Vancouver British Columbia V6T 1Z1 Canada

Department of Physics and Astronomy University of Waterloo Waterloo Ontario N2L 3G1 Canada

Department of Physics and Astronomy University of Tennessee Knoxville Tennessee 37996 USA

Center for Nanophase Materials Sciences Oak Ridge National Laboratory Oak Ridge TN 37831 USA

Funding

Office of Science · National Science Foundation

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