journal article·2024-02Open access

CO2‐Induced Spin‐Lattice Coupling for Strong Magnetoelectric Materials

Bo Gao, Song Xu, Qun Xu

Advanced Science· Volume 11· Issue 5

Abstract

Abstract The preparation of 2D magnetoelectric (ME) nanomaterials with strong ME coupling is crucial for the fast reading and writing processes in the next generation of storage devices. Herein, 2D BaTiO3 (BTO)‐CoFe2O4 (CFO) ME nanocomposites are prepared through a substrate‐free coupling strategy using supercritical CO2. Such 2D BTO‐CFO with strong coupling is built through alternating in‐plane and out‐of‐plane epitaxy stacking, leading to remarkable mutual biaxial strain effects for spin‐lattice coupling. As a results, such strain effect significantly enhances the ferroelectricity of BTO and the ferrimagnetism of CFO, where an unexceptionally high ME coupling coefficient of (325.8 mV cm−1 Oe−1) is obtained for the BTO‐CFO nanocomposites.
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Research context

OpenAlex topics: Multiferroics and related materials · Ferroelectric and Piezoelectric Materials · Advanced Condensed Matter Physics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

College of Materials Science & Engineering Zhengzhou University Zhengzhou 450001 P. R. China

Institute of Advanced Technology Zhengzhou University Zhengzhou 450001 P. R. China

Funding

National Natural Science Foundation of China

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