journal article·2024-08Open access

Ultrafast Opto‐Electronic and Thermal Tuning of Third‐Harmonic Generation in a Graphene Field Effect Transistor

Omid Ghaebi, Sebastian Klimmer, Nele Tornow, Niels Buijssen, Takashi Taniguchi, Kenji Watanabe, Andrea Tomadin, Habib Rostami, Giancarlo Soavi

Advanced Science· Volume 11· Issue 31

Abstract

Abstract Graphene is a unique platform for tunable opto‐electronic applications thanks to its linear band dispersion, which allows electrical control of resonant light‐matter interactions. Tuning the nonlinear optical response of graphene is possible both electrically and in an all‐optical fashion, but each approach involves a trade‐off between speed and modulation depth. Here, lattice temperature, electron doping, and all‐optical tuning of third‐harmonic generation are combined in a hexagonal boron nitride‐encapsulated graphene opto‐electronic device and demonstrate up to 85% modulation depth along with gate‐tunable ultrafast dynamics. These results arise from the dynamic changes in the transient electronic temperature combined with Pauli blocking induced by the out‐of‐equilibrium chemical potential. The work provides a detailed description of the transient nonlinear optical and electronic response of graphene, which is crucial for the design of nanoscale and ultrafast optical modulators, detectors, and frequency converters.
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Research context

OpenAlex topics: Advanced Fiber Laser Technologies · Photonic and Optical Devices · Mechanical and Optical Resonators

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Solid State Physics Friedrich Schiller University Jena 07743 Jena Germany

ARC Centre of Excellence for Transformative Meta‐Optical Systems Department of Electronic Materials Engineering Research School of Physics The Australian National University Canberra ACT 2601 Australia

Research Center for Materials Nanoarchitectonics National Institute for Materials Science 1‐1 Namiki Tsukuba 305‐0044 Japan

Research Center for Electronic and Optical Materials National Institute for Materials Science 1‐1 Namiki Tsukuba 305‐0044 Japan

Dipartimento di Fisica Università di Pisa Largo Bruno Pontecorvo 3 Pisa 56127 Italy

Department of Physics University of Bath Claverton Down Bath BA2 7AY UK

Abbe Center of Photonics Friedrich Schiller University Jena 07743 Jena Germany

Funding

European Commission · Vetenskapsrådet · Deutsche Forschungsgemeinschaft

References (51)

Show source-provided references
1. 10.1002/lpor.20210072610.1002/lpor.202100726 ↗
2. 10.1038/s41566-020-00728-010.1038/s41566-020-00728-0 ↗
3. 10.1038/s41586-022-05393-710.1038/s41586-022-05393-7 ↗
4. 10.1038/s41566-021-00859-y10.1038/s41566-021-00859-y ↗
5. 10.1021/acs.nanolett.0c0297210.1021/acs.nanolett.0c02972 ↗
6. 10.1038/nnano.2015.7310.1038/nnano.2015.73 ↗
7. 10.1002/smll.20190634710.1002/smll.201906347 ↗
8. 10.1038/s41565-018-0145-810.1038/s41565-018-0145-8 ↗
9. 10.1021/acsphotonics.9b0092810.1021/acsphotonics.9b00928 ↗
10. 10.1038/s41586-018-0508-110.1038/s41586-018-0508-1 ↗
11. 10.1021/acs.nanolett.0c0217410.1021/acs.nanolett.0c02174 ↗
12. 10.1038/s41467-022-30901-810.1038/s41467-022-30901-8 ↗
13. 10.1126/sciadv.abq824610.1126/sciadv.abq8246 ↗
14. 10.1002/smll.20230112610.1002/smll.202301126 ↗
15. P.Herrmann S.Klimmer T.Weickhardt A.Papavasileiou K.Mosina Z.Sofer I.Paradisanos D.Kartashov G.Soavi(Preprint) arXiv:2310.16549 submitted: October2023.
16. 10.1103/PhysRevB.82.12541110.1103/PhysRevB.82.125411 ↗
17. 10.1063/1.327574010.1063/1.3275740 ↗
18. 10.1103/PhysRevB.85.12141310.1103/PhysRevB.85.121413 ↗
19. 10.1021/nl400451410.1021/nl4004514 ↗
20. 10.1103/PhysRevLett.122.04740110.1103/PhysRevLett.122.047401 ↗
21. 10.1038/s41566-018-0175-710.1038/s41566-018-0175-7 ↗
22. 10.1038/s41565-020-00808-w10.1038/s41565-020-00808-w ↗
23. 10.1103/PhysRevB.87.12140610.1103/PhysRevB.87.121406 ↗
24. 10.1103/PhysRevX.3.02101410.1103/PhysRevX.3.021014 ↗
25. 10.1063/1.326496410.1063/1.3264964 ↗
26. 10.1021/nn901703e10.1021/nn901703e ↗
27. 10.1063/1.508864110.1063/1.5088641 ↗
28. 10.1038/s41565-017-0008-810.1038/s41565-017-0008-8 ↗
29. 10.1088/2053-1583/abf08d10.1088/2053-1583/abf08d ↗
30. 10.1021/acsnano.0c1086410.1021/acsnano.0c10864 ↗
31. 10.1038/s41467-018-07558-310.1038/s41467-018-07558-3 ↗
32. 10.1364/OL.12.00055210.1364/OL.12.000552 ↗
33. 10.1038/srep1684110.1038/srep16841 ↗
34. 10.1038/nphys256410.1038/nphys2564 ↗
35. 10.1038/ncomms298710.1038/ncomms2987 ↗
36. 10.1103/PhysRevB.88.03543010.1103/PhysRevB.88.035430 ↗
37. 10.1039/D0NR09166A10.1039/D0NR09166A ↗
38. 10.1021/acsnano.1c0493710.1021/acsnano.1c04937 ↗
39. 10.1103/PhysRevB.93.16141110.1103/PhysRevB.93.161411 ↗
40. 10.1017/CBO978051161991510.1017/CBO9780511619915 ↗
41. 10.1103/PhysRevB.88.03543010.1103/PhysRevB.88.035430 ↗
42. 10.1103/PhysRevLett.112.25740110.1103/PhysRevLett.112.257401 ↗
43. 10.1103/PhysRevB.87.08531910.1103/PhysRevB.87.085319 ↗
44. 10.1002/adom.20200044110.1002/adom.202000441 ↗
45. 10.1103/PhysRevB.93.04540710.1103/PhysRevB.93.045407 ↗
46. 10.1038/s41467-024-46642-910.1038/s41467-024-46642-9 ↗
47. 10.1021/acsphotonics.1c0046610.1021/acsphotonics.1c00466 ↗
48. D.Popa D.Viola G.Soavi B.Fu L.Lombardi S.Hodge D.Polli T.Scopigno G.Cerullo A. C.Ferrari inCLEO: QELS_Fundamental Science JTu5A–2 Optica Publishing Group Washington D.C.2017.10.1364/CLEO_AT.2017.JTu5A.2 ↗
49. 10.1038/s41566-023-01195-z10.1038/s41566-023-01195-z ↗
50. 10.1038/s41566-022-01067-y10.1038/s41566-022-01067-y ↗
51. 10.1002/smll.20190656310.1002/smll.201906563 ↗