journal article·2025-05-28

Cost-Efficient Deterministic Engineering of Single Photon Emitters in Two-Dimensional Materials

Sanja Djurdjić Mijin, Ismael dePedro-Embid, Nikita Panov, Eva Hemmer, Snežana Lazić

ACS Applied Materials & Interfaces· Volume 17· Issue 21
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Abstract

Two-dimensional materials have recently emerged as promising candidates for quantum light emission. Their tunable bandgaps, layer-dependent excitonic properties, and strong confinement of charge carriers provide a versatile platform for manipulating and controlling quantum states. Several approaches─such as strain engineering, defect engineering and surface functionalization─have been explored to induce single-photon emitters in these materials. In this work, we present a practical and cost-efficient methodology for deterministic strain engineering of single-photon emitters within thin flakes of GaSe. Our approach utilizes optically active microparticles with a distinctive bipyramidal shape, whose emission does not interfere optically with that of GaSe. The results show strong agreement with previous studies on strain-induced single-photon sources in multilayer GaSe, demonstrating that the proposed technique is a promising platform for generating nonclassical light emission in layered materials. Compared to other local strain engineering techniques for single-photon sources in two-dimensional materials, our method offers greater accessibility and lower cost, making it feasible for implementation in most laboratories performing the experimental research in the field. This increased accessibility can help advance the understanding of two-dimensional semiconductor systems and their potential applications in nanophotonics and quantum light technologies.
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Research context

OpenAlex topics: Nanowire Synthesis and Applications · Advanced Semiconductor Detectors and Materials · 2D Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Departamento de Física de Materiales, Facultad de Ciencias

Universidad Autónoma de Madrid (UAM)

Institute of Physics Belgrade, University of Belgrade, Pregrevica 118, 11080 Belgrade, Serbia

Paul-Drude-Institut für Festkörperelektronik, Leibniz-Institut im Forschungsverbund Berlin e.V., Hausvogteiplatz 5−7, 10117 Berlin, Germany

Nanomaterials for Bioimaging Group (nanoBIG), Departamento de Física de Materiales, Facultad de Ciencias

Department of Chemistry and Biomolecular Sciences

University of Ottawa

Instituto Universitario de Ciencia de Materiales “Nicolás Cabrera” (INC) and Condensed Matter Physics Center (IFIMAC), UAM

Funding

Ministerio de Ciencia, Innovaci?n y Universidades · NATO Science for Peace and Security Programme

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