journal article·2025-03-26Open access

Interfacial Spin–Orbit-Coupling-Induced Strong Spin-to-Charge Conversion at an All-Oxide Ferromagnetic/Quasi-Two-Dimensional Electron Gas Interface

Mi-Jin Jin, Guang Yang, Doo-Seung Um, Jacob Linder, Jason W.A. Robinson

ACS Applied Materials & Interfaces· Volume 17· Issue 12

Abstract

High Resolution Image Download MS PowerPoint Slide Functional oxides and hybrid structures with interfacial spin–orbit coupling and the Rashba–Edelstein effect (REE) are promising materials systems for thermal tolerance spintronic device applications. Here, we demonstrate efficient spin-to-charge conversion through enhanced interfacial spin–orbit coupling at the all-oxide interface of La 1– x Ca x MnO 3 with quasi-two-dimensional (quasi-2D) SrTiO 3 (LCMO/STO). The quasi-2D interface is generated via oxygen vacancies at the STO surface. We obtain a spin-to-charge conversion efficiency of θ ∥ ≈ 2.32 ± 1.3 nm, most likely originating from the inverse REE, which is relatively large versus all-metallic spin-to-charge conversion materials systems. The results highlight that the LCMO/STO 2D electron gas is a potential platform for spin-based memory and transistor applications.
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Research context

OpenAlex topics: Electronic and Structural Properties of Oxides · ZnO doping and properties · Magnetic properties of thin films

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Affiliations

Center for Multidimensional Carbon Materials (CMCM)

Institute for Basic Science (IBS)

Department of Materials Science & Metallurgy, University of Cambridge, 27 Charles Babbage Road, Cambridge CB3 0FS, United Kingdom

School of Integrated Circuit Science and Engineering

Beihang University

Department of Electronic Engineering

Jeju National University (JNU)

Center for Quantum Spintronics, Department of Physics

Norwegian University of Science and Technology

Funding

Engineering and Physical Sciences Research Council · Norges Forskningsr?d · National Research Foundation of Korea · Institute for Basic Science

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