journal article·2024-10-09Open access

High-Performance Red Transparent Quantum Dot Light-Emitting Diodes via Fully Solution-Processed MXene/Ag NWs Top Electrode

Daojian Su, Ting Ding, Peili Gao, Hang Liu, Yinman Song, Guoqiang Yuan, Xin He, Fanyuan Meng, Shuangpeng Wang

ACS Applied Materials & Interfaces· Volume 16· Issue 40

Abstract

High Resolution Image Download MS PowerPoint Slide The integration of high-performance transparent top electrodes with the functional layers of transparent quantum dot light-emitting diodes (T-QLEDs) poses a notable challenge. This study presents a composite transparent top electrode composed of MXene and Ag NWs. The composite electrode demonstrates exceptional transparency (84.6% at 620 nm) and low sheet resistance (16.07 Ω sq –1 ), rendering it suitable for integration into T-QLEDs. The inclusion of MXene nanosheets in the composite electrode serves a dual role: adjusting the work function to enhance electron injection efficiency and enhancing the interface between Ag NWs and the emissive layer, thereby mitigating the common issue of interfacial resistance in conventional transparent electrodes. This strategic amalgamation results in notable improvements in device performance, yielding a maximum current efficiency of 23.12 cd A –1, an external quantum efficiency of 13.98%, and a brightness of 21,015 cd m –2 . These performance metrics surpass those achieved by T-LEDs employing pristine Ag NW electrodes. This study offers valuable insights into T-QLED device advancement and provides a promising approach for transparent electrode fabrication in optoelectronic applications.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Quantum Dots Synthesis And Properties · Nanocluster Synthesis and Applications · Gold and Silver Nanoparticles Synthesis and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Applied Physics and Materials, Wuyi University, Jiangmen 529020, P. R. China

Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macau 999078, P. R. China

Jiangmen Key Laboratory of Micro-Nano Functional Materials and Devices, Jiangmen 529020, P. R. China

Funding

Basic and Applied Basic Research Foundation of Guangdong Province · Department of Education of Guangdong Province · Wuyi University-Hong Kong-Macau Joint Research and Development Fund

References (54)

Show source-provided references
1. 10.1038/s41377-020-0341-910.1038/s41377-020-0341-9 ↗
2. 10.1002/adma.20210469010.1002/adma.202104690 ↗
3. 10.1016/j.cej.2021.13085810.1016/j.cej.2021.130858 ↗
4. 10.1002/adma.20221038510.1002/adma.202210385 ↗
5. 10.1002/anie.20090305310.1002/anie.200903053 ↗
6. 10.3402/nano.v1i0.520210.3402/nano.v1i0.5202 ↗
7. 10.1002/adfm.20170061010.1002/adfm.201700610 ↗
8. 10.1002/adfm.20210638710.1002/adfm.202106387 ↗
9. 10.1002/adma.20210815010.1002/adma.202108150 ↗
10. 10.1002/adma.20080325610.1002/adma.200803256 ↗
11. 10.1021/acsnano.6b0450610.1021/acsnano.6b04506 ↗
12. 10.1038/s41467-020-18110-710.1038/s41467-020-18110-7 ↗
13. 10.1002/adma.20210469010.1002/adma.202104690 ↗
14. 10.1038/s41566-022-00960-w10.1038/s41566-022-00960-w ↗
15. 10.1038/s41528-022-00234-z10.1038/s41528-022-00234-z ↗
16. 10.1002/adma.20170327910.1002/adma.201703279 ↗
17. 10.1021/acsaelm.0c0033210.1021/acsaelm.0c00332 ↗
18. 10.1088/1361-6528/ab4dcd10.1088/1361-6528/ab4dcd ↗
19. 10.1002/adma.20230332910.1002/adma.202303329 ↗
20. 10.1021/acsnano.7b0786710.1021/acsnano.7b07867 ↗
21. 10.1021/acsami.8b1894010.1021/acsami.8b18940 ↗
22. 10.1007/s40843-019-9437-910.1007/s40843-019-9437-9 ↗
23. 10.1002/adom.20210038910.1002/adom.202100389 ↗
24. 10.1021/acsami.2c0436910.1021/acsami.2c04369 ↗
25. 10.1021/acsami.2c0964510.1021/acsami.2c09645 ↗
26. 10.1039/C8TC06121A10.1039/C8TC06121A ↗
27. 10.1038/s41528-021-00106-y10.1038/s41528-021-00106-y ↗
28. 10.1364/PRJ.42475010.1364/PRJ.424750 ↗
29. 10.1039/C5TC04223B10.1039/C5TC04223B ↗
30. 10.1002/adom.20210240410.1002/adom.202102404 ↗
31. 10.1021/acsami.7b0202610.1021/acsami.7b02026 ↗
32. 10.1021/acsami.9b0596910.1021/acsami.9b05969 ↗
33. 10.1021/acsami.0c1546910.1021/acsami.0c15469 ↗
34. 10.31635/ccschem.020.20200040210.31635/ccschem.020.202000402 ↗
35. 10.1002/adfm.20230846810.1002/adfm.202308468 ↗
36. 10.1021/acsnano.2c1118010.1021/acsnano.2c11180 ↗
37. 10.1038/s41467-021-21435-610.1038/s41467-021-21435-6 ↗
38. 10.1016/j.cej.2020.12719210.1016/j.cej.2020.127192 ↗
39. 10.1002/advs.20200156210.1002/advs.202001562 ↗
40. 10.1002/adom.20220180210.1002/adom.202201802 ↗
41. 10.1021/acsami.9b0411310.1021/acsami.9b04113 ↗
42. 10.1021/acsnano.2c0151410.1021/acsnano.2c01514 ↗
43. 10.1021/acsaelm.0c0033210.1021/acsaelm.0c00332 ↗
44. 10.1007/s40820-021-00664-w10.1007/s40820-021-00664-w ↗
45. 10.1002/adfm.20210130210.1002/adfm.202101302 ↗
46. 10.1039/D0NR01885F10.1039/D0NR01885F ↗
47. 10.1002/adom.20210038910.1002/adom.202100389 ↗
48. 10.1002/smll.20230458010.1002/smll.202304580 ↗
49. 10.1038/s41467-019-08749-210.1038/s41467-019-08749-2 ↗
50. 10.1016/j.mejo.2022.10538810.1016/j.mejo.2022.105388 ↗
51. 10.1021/acsami.1c1305210.1021/acsami.1c13052 ↗
52. 10.1039/C7NR05472F10.1039/C7NR05472F ↗
53. 10.1002/advs.20180054910.1002/advs.201800549 ↗
54. 10.1002/adma.20200617810.1002/adma.202006178 ↗