journal article·2023-08-23

Room-Temperature, Homogeneous, Single-Step, and Large-Scale Synthesis of Perovskite Nanoplatelets for Blue Light-Emitting Diodes

Ju-Hyun Yoo, Sungjin Kim, Hyeokjung Lee, Cheolmin Park, Tae-Woo Lee, Jin-Woo Park

ACS Applied Materials & Interfaces· Volume 15· Issue 33
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Abstract

Inorganic perovskite nanocrystals (IPNCs) have attracted considerable attention due to their excellent optoelectronic properties. However, problems arise from anion migration during the preparation of a blue light-emitting diode (LED), and only small-scale syntheses have been conducted on a laboratory scale. By using only Br as the anion here, CsPbBr 3 was synthesized in the form of nanoplatelets to eliminate the effects of anion migration and to prepare an inorganic perovskite nanoplatelet (IPNPL) emitting blue light. In addition, the synthesis was performed under ambient conditions at room temperature, and the synthetic process was shortened to enable large-scale synthesis. We used a 1 L bottle for large-scale synthesis, and a photoluminescence quantum yield (PLQY) of 78% was observed at 460 nm. We fabricated LEDs by using IPNPLs, and we observed an electroluminescence peak at 461 nm. The developed synthetic method is expected to pave the way for commercialization of IPNCs and the next-generation display market.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Quantum Dots Synthesis And Properties · Organic Light-Emitting Diodes Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Materials Science and Engineering, Yonsei University, Seoul 03722, Republic of Korea

Department of Materials Science and Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea

School of Chemical and Biological Engineering, Institute of Engineering Research, Research Institute of Advanced Materials, Soft Foundry, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea

Funding

National Research Foundation of Korea

References (38)

Show source-provided references
1. 10.1002/adfm.20160010910.1002/adfm.201600109 ↗
2. 10.1002/adma.20160388510.1002/adma.201603885 ↗
3. 10.1039/C8CS00740C10.1039/C8CS00740C ↗
4. 10.1016/j.nanoen.2018.06.05610.1016/j.nanoen.2018.06.056 ↗
5. 10.1126/science.aam709310.1126/science.aam7093 ↗
6. 10.1002/adfm.20211189410.1002/adfm.202111894 ↗
7. 10.1016/j.sse.2019.10774910.1016/j.sse.2019.107749 ↗
8. 10.1038/s41566-020-00732-410.1038/s41566-020-00732-4 ↗
9. 10.1016/j.mser.2018.12.00110.1016/j.mser.2018.12.001 ↗
10. 10.1016/j.matdes.2019.10810010.1016/j.matdes.2019.108100 ↗
11. 10.1021/acsnano.5b0819310.1021/acsnano.5b08193 ↗
12. 10.1002/adma.20180199610.1002/adma.201801996 ↗
13. 10.1021/acs.nanolett.5b0298510.1021/acs.nanolett.5b02985 ↗
14. 10.1002/adma.20220085410.1002/adma.202200854 ↗
15. 10.1038/s41565-020-0714-510.1038/s41565-020-0714-5 ↗
16. 10.1021/acs.chemmater.8b0299910.1021/acs.chemmater.8b02999 ↗
17. 10.1021/acs.nanolett.8b0219010.1021/acs.nanolett.8b02190 ↗
18. 10.1021/acsenergylett.0c0265110.1021/acsenergylett.0c02651 ↗
19. 10.1038/s41586-022-05486-310.1038/s41586-022-05486-3 ↗
20. 10.1021/acsenergylett.0c0047110.1021/acsenergylett.0c00471 ↗
21. 10.1088/1361-648X/ac00db10.1088/1361-648X/ac00db ↗
22. 10.1021/nl504877910.1021/nl5048779 ↗
23. 10.1038/s41563-020-0784-710.1038/s41563-020-0784-7 ↗
24. 10.1002/smtd.20190019610.1002/smtd.201900196 ↗
25. 10.1021/acsnano.5b0115410.1021/acsnano.5b01154 ↗
26. 10.1021/acs.nanolett.5b0240410.1021/acs.nanolett.5b02404 ↗
27. 10.1021/jacs.5b0560210.1021/jacs.5b05602 ↗
28. 10.1039/C6CC01500J10.1039/C6CC01500J ↗
29. 10.1039/C8NR09885A10.1039/C8NR09885A ↗
30. 10.1016/j.jlumin.2019.03.01410.1016/j.jlumin.2019.03.014 ↗
31. 10.1021/acs.chemmater.6b0224110.1021/acs.chemmater.6b02241 ↗
32. 10.1021/acs.chemmater.7b0138410.1021/acs.chemmater.7b01384 ↗
33. 10.1002/adma.20210710510.1002/adma.202107105 ↗
34. 10.1002/adfm.20210868710.1002/adfm.202108687 ↗
35. 10.1021/jacs.5b1212410.1021/jacs.5b12124 ↗
36. 10.1021/acsenergylett.8b0102510.1021/acsenergylett.8b01025 ↗
37. 10.1039/C8NR09349K10.1039/C8NR09349K ↗
38. 10.1016/j.nanoen.2018.03.01910.1016/j.nanoen.2018.03.019 ↗