journal article·2024-02-14Open access

Asymmetric Triphenylethylene-Based Hole Transporting Materials for Highly Efficient Perovskite Solar Cells

Julius Petrulevicius, Yi Yang, Cheng Liu, Matas Steponaitis, Egidijus Kamarauskas, Maryte Daskeviciene, Abdulaziz S. R. Bati, Tadas Malinauskas, Vygintas Jankauskas, Kasparas Rakstys, Mercouri G. Kanatzidis, Edward H. Sargent, Vytautas Getautis

Abstract

Molecular hole-transporting materials (HTMs) having triphenylethylene central core were designed, synthesized, and employed in perovskite solar cell (PSC) devices. The synthesized HTM derivatives were obtained in a two- or three-step synthetic procedure, and their characteristics were analyzed by various thermoanalytical, optical, photophysical, and photovoltaic techniques. The most efficient PSC device recorded a 23.43% power conversion efficiency. Furthermore, the longevity of the device employing V1509 HTM surpassed that of PSC with state-of-art spiro-OMeTAD as the reference HTM.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Conducting polymers and applications · Organic Light-Emitting Diodes Research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Organic Chemistry, Kaunas University of Technology, Radvilenu pl. 19, Kaunas 50254, Lithuania

Department of Chemistry, Northwestern University, 2145 Sheridan Rd, Evanston, Illinois 60208, United States

Institute of Chemical Physics Vilnius University, Sauletekio al. 3, Vilnius 10257, Lithuania

Department of Electrical and Computer Engineering, Northwestern University, 2145 Sheridan Rd, Evanston, Illinois 60208, United States

Funding

King Abdullah University of Science and Technology · Office of Naval Research · HORIZON EUROPE Climate, Energy and Mobility

References (37)

Show source-provided references
1. 10.1038/s41586-021-03285-w10.1038/s41586-021-03285-w ↗
2. 10.1002/aenm.20220097510.1002/aenm.202200975 ↗
3. 10.1126/sciadv.abo742210.1126/sciadv.abo7422 ↗
4. 10.1021/acsenergylett.2c0150610.1021/acsenergylett.2c01506 ↗
5. 10.1038/s41598-020-63674-510.1038/s41598-020-63674-5 ↗
6. 10.1038/s41467-021-22049-810.1038/s41467-021-22049-8 ↗
7. 10.1038/s41560-019-0529-510.1038/s41560-019-0529-5 ↗
8. 10.1021/acsaem.1c0237510.1021/acsaem.1c02375 ↗
9. 10.3389/fchem.2020.0072510.3389/fchem.2020.00725 ↗
10. 10.1002/chem.20180144110.1002/chem.201801441 ↗
11. 10.1039/C8TC02242A10.1039/C8TC02242A ↗
12. 10.1038/s41467-018-07255-110.1038/s41467-018-07255-1 ↗
13. 10.1016/j.chempr.2017.03.01110.1016/j.chempr.2017.03.011 ↗
14. 10.1002/adfm.20180709410.1002/adfm.201807094 ↗
15. 10.1021/acsami.0c0631810.1021/acsami.0c06318 ↗
16. 10.1021/acsami.5b0466210.1021/acsami.5b04662 ↗
17. 10.1039/C7TA04762B10.1039/C7TA04762B ↗
18. 10.1039/C7CC04606E10.1039/C7CC04606E ↗
19. 10.1002/cssc.20170097310.1002/cssc.201700973 ↗
20. 10.1039/C7CC08985F10.1039/C7CC08985F ↗
21. 10.1021/jacs.7b1089810.1021/jacs.7b10898 ↗
22. 10.1039/C9CC09901H10.1039/C9CC09901H ↗
23. 10.1039/D1CP05503H10.1039/D1CP05503H ↗
24. 10.1002/anie.20191502210.1002/anie.201915022 ↗
25. 10.1021/acsenergylett.2c0068410.1021/acsenergylett.2c00684 ↗
26. 10.1021/jacs.5b1107610.1021/jacs.5b11076 ↗
27. 10.1039/C5RA06876B10.1039/C5RA06876B ↗
28. 10.1039/C8TC04231D10.1039/C8TC04231D ↗
29. 10.1002/adfm.20170435110.1002/adfm.201704351 ↗
30. 10.1021/acsami.1c0589010.1021/acsami.1c05890 ↗
31. 10.1039/D0SE01062F10.1039/D0SE01062F ↗
32. 10.1021/acs.chemmater.9b0070210.1021/acs.chemmater.9b00702 ↗
33. 10.1021/nn204296b10.1021/nn204296b ↗
34. 10.1039/D0TA08452B10.1039/D0TA08452B ↗
35. 10.1002/anie.20211320710.1002/anie.202113207 ↗
36. 10.1021/acsenergylett.9b0226210.1021/acsenergylett.9b02262 ↗
37. 10.1038/s41586-021-03285-w10.1038/s41586-021-03285-w ↗