journal article·2017-07-12

Quantum Dots-Facilitated Printing of ZnO Nanostructure Photodetectors with Improved Performance

Brent Cook, Qingfeng Liu, Maogang Gong, Dan Ewing, Matthew Casper, Alex Stramel, Judy Wu

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Abstract

A nanocomposite ink composed of zinc oxide precursor (ZnOPr) and crystalline ZnO quantum dots (ZnOPrQDs) has been explored for printing high-performance ultraviolet (UV) photodetectors. The performance of the devices has been compared with their counterparts' printed from ZnOPr ink without ZnO QDs. Remarkably, higher UV photoresponsivity of 383.6 A/W and the on/off ratio of 2470 are observed in the former, which are significantly better than 14.7 A/W and 949 in the latter. The improved performance is attributed to the increased viscosity in the nanocomposite ink to enable a nanoporous structure with improved crystallinity and surface-to-volume ratio. This is key to enhanced surface electron-depletion effect for higher UV responsivity and on/off ratio. In addition, the QD-assisted printing provides a simple and robust method for printing high-performance optoelectronics and sensors.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: ZnO doping and properties · Gas Sensing Nanomaterials and Sensors · Ga2O3 and related materials

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics and Astronomy, University of Kansas, Lawrence, Kansas 66045, United States

Department of Energy’s National Security Campus, Kansas City, Missouri 64147, United States

Funding

Army Research Office · U.S. Department of Energy · Division of Materials Research

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