journal article·2022-08-10

Multistrategy Preparation of Efficient and Stable Environment-Friendly Lead-Based Perovskite Solar Cells

Huan Bi, Gaoyi Han, Mengna Guo, Chao Ding, Hanjun Zou, Qing Shen, Shuzi Hayase, Wenjing Hou

ACS Applied Materials & Interfaces· Volume 14· Issue 31
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Abstract

Perovskite solar cells (PSCs) have achieved huge success in power conversion efficiency (PCE) and stability. However, further improving the PCE of PSCs and stability is still a big challenge. Here, we attempt to improve the PCE and stability of PSCs using a functional additive named 3-mercaptopropyltriethoxysilane (SiSH) in the perovskite antisolvent. It is revealed that SiSH can release the stress in the film, reduce the defects, and inhibit lithium-ion migration and lead leakage. As a result, the target device achieves an efficiency enhancement from 20.80 to 22.42% as compared to the control device. Meanwhile, device stability is ameliorated after SiSH modification. Furthermore, new adsorbents are used to treat the leaked lead to make it comply with safe drinking water standards. This work provides an idea for developing multifunctional antisolvent additives and adsorbents for high PCE, long stability, and environment-friendly Pb-based PSCs.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Conducting polymers and applications · Advanced battery technologies research

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Graduate School of Informatics and Engineering, The University of Electro-Communication, Tokyo 182-8585, Japan

Institute of Molecular Science, Key Laboratory of Materials for Energy Conversion and Storage of Shanxi Province, Shanxi University, Taiyuan 030006, P. R. China

Analytical and Testing Center, Chongqing University, Chongqing 401331, P. R. China

Funding

Natural Science Foundation of Shanxi Province · Ministry of Education, Culture, Sports, Science and Technology · National Natural Science Foundation of China · State Key Laboratory of Quantum Optics and Quantum Optics Devices. Institute of Opto-Electronics, Shanxi University · Scientific and Technological Innovation Programs of Higher Education Institutions in Shanxi

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