journal article·2018-05-09

Sub-Band Gap Turn-On Near-Infrared-to-Visible Up-Conversion Device Enabled by an Organic–Inorganic Hybrid Perovskite Photovoltaic Absorber

By Hyeonggeun Yu, Yuanhang Cheng, Menglin Li, Sai-Wing Tsang, Franky So

ACS Applied Materials & Interfaces· Volume 10· Issue 18
Publisher page

Abstract

Direct integration of an infrared (IR) photodetector with an organic light-emitting diode (OLED) enables low-cost, pixel-free IR imaging. However, the operation voltage of the resulting IR-to-visible up-conversion is large because of the series device architecture. Here, we report a low-voltage near-IR (NIR)-to-visible up-conversion device using formamidinium lead iodide as a NIR absorber integrated with a phosphorescent OLED. Because of the efficient photocarrier injection from the hybrid perovskite layer to the OLED, we observed a sub-band gap turn-on of the OLED under NIR illumination. The device showed a NIR-to-visible up-conversion efficiency of 3% and a luminance on/off ratio of 103 at only 5 V. Finally, we demonstrate pixel-free NIR imaging using the up-conversion device.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Ga2O3 and related materials · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Materials Science and Engineering, North Carolina State University, Raleigh, North Carolina 27606, United States

Department of Physics and Materials Science, City University of Hong Kong, Hong Kong SAR, P. R. China

Funding

Nanoholdings LLC.

References (32)

Show source-provided references
1. 10.1038/nnano.2009.29410.1038/nnano.2009.294 ↗
2. 10.1038/nbt99410.1038/nbt994 ↗
3. 10.1038/nphoton.2006.510.1038/nphoton.2006.5 ↗
4. 10.1117/12.47885810.1117/12.478858 ↗
5. 10.1038/nphoton.2015.27010.1038/nphoton.2015.270 ↗
6. 10.1021/acsphotonics.6b0096410.1021/acsphotonics.6b00964 ↗
7. 10.1002/adma.20090331210.1002/adma.200903312 ↗
8. 10.1021/nl200704h10.1021/nl200704h ↗
9. 10.1038/srep0594610.1038/srep05946 ↗
10. 10.1063/1.271000310.1063/1.2710003 ↗
11. 10.1002/adma.20120058710.1002/adma.201200587 ↗
12. 10.1016/j.orgel.2011.09.00310.1016/j.orgel.2011.09.003 ↗
13. 10.1039/c5ee03874j10.1039/c5ee03874j ↗
14. 10.1126/science.aaf806010.1126/science.aaf8060 ↗
15. 10.1002/pip.290910.1002/pip.2909 ↗
16. 10.1038/ncomms640410.1038/ncomms6404 ↗
17. 10.1038/ncomms972410.1038/ncomms9724 ↗
18. 10.1002/adma.20140511610.1002/adma.201405116 ↗
19. 10.1038/nature1413310.1038/nature14133 ↗
20. 10.1021/jp411112k10.1021/jp411112k ↗
21. 10.1002/smll.20140276710.1002/smll.201402767 ↗
22. 10.1021/ja503325910.1021/ja5033259 ↗
23. 10.1038/ncomms770010.1038/ncomms7700 ↗
24. 10.1063/1.324399110.1063/1.3243991 ↗
25. 10.1002/adma.20150296910.1002/adma.201502969 ↗
26. 10.1038/ncomms458610.1038/ncomms4586 ↗
27. 10.1038/ncomms923810.1038/ncomms9238 ↗
28. 10.1002/adma.20150009910.1002/adma.201500099 ↗
29. 10.1063/1.12570110.1063/1.125701 ↗
30. 10.1063/1.300038210.1063/1.3000382 ↗
31. 10.1016/j.sse.2010.10.01810.1016/j.sse.2010.10.018 ↗
32. 10.1021/acsphotonics.5b0016410.1021/acsphotonics.5b00164 ↗