journal article·2020-04-01

Improved Performance for Thermally Evaporated Perovskite Light-Emitting Devices via Defect Passivation and Carrier Regulation

Kuifeng Jia, Li Song, Yongsheng Hu, Xiaoyang Guo, Xingyuan Liu, Chong Geng, Shu Xu, Ruiting Fan, Lixin Huang, Nannan Luan, Wengang Bi

ACS Applied Materials & Interfaces· Volume 12· Issue 13
Publisher page

Abstract

Efficient inorganic perovskite light-emitting devices (PeLEDs) with a vacuum-deposited CsPbBr3 emission layer were realized by introducing an ultrathin 2-phenylethanamine bromide interlayer. The PEA+ cations not only passivated the nonradiative defects by terminating on the CsPbBr3 surface but also regulated the charge transport to balance the hole and electron transport. Consequently, the PeLEDs exhibit significantly promoted performance with a turn-on voltage of 3 V, a maximum current efficiency of 14.64 cd A–1, and an external quantum efficiency of 4.10%. Our work would provide instructive guidance for realizing efficient PeLEDs based on a vacuum processing method via focusing on the interface modification between the perovskite layer and the carrier transport layer.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Chalcogenide Semiconductor Thin Films · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Tianjin Key Laboratory of Electronic Materials and Devices, School of Electronics and Information Engineering, Hebei University of Technology, 5340 Xiping Road, Tianjin 300401, P. R. China

State Key Laboratory of Luminescence and Applications, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China

Funding

Natural Science Foundation of Hebei Province · Natural Science Foundation of Tianjin City · Department of Science and Technology of Jilin Province · National Natural Science Foundation of China · State Key Laboratory of Luminescence and Applications

References (38)

Show source-provided references
1. 10.1038/nphoton.2016.18510.1038/nphoton.2016.185 ↗
2. 10.1002/aenm.20160115610.1002/aenm.201601156 ↗
3. 10.1021/acsnano.6b0391610.1021/acsnano.6b03916 ↗
4. 10.1002/adma.20160062610.1002/adma.201600626 ↗
5. 10.1021/acsenergylett.7b0096710.1021/acsenergylett.7b00967 ↗
6. 10.1021/jacs.7b1043010.1021/jacs.7b10430 ↗
7. 10.1038/lsa.2016.5610.1038/lsa.2016.56 ↗
8. 10.1038/nphoton.2016.4110.1038/nphoton.2016.41 ↗
9. 10.1038/lsa.2017.2310.1038/lsa.2017.23 ↗
10. 10.1002/adma.20160312610.1002/adma.201603126 ↗
11. 10.1002/adma.20180025110.1002/adma.201800251 ↗
12. 10.1021/acsami.8b0743810.1021/acsami.8b07438 ↗
13. 10.1038/nnano.2014.14910.1038/nnano.2014.149 ↗
14. 10.1038/s41586-018-0576-210.1038/s41586-018-0576-2 ↗
15. 10.1038/s41586-018-0575-310.1038/s41586-018-0575-3 ↗
16. 10.1038/s41566-018-0260-y10.1038/s41566-018-0260-y ↗
17. 10.1021/acsnano.7b0785610.1021/acsnano.7b07856 ↗
18. 10.1021/acsami.8b1341810.1021/acsami.8b13418 ↗
19. 10.1039/c7tc04631f10.1039/c7tc04631f ↗
20. 10.1021/acs.cgd.6b0076410.1021/acs.cgd.6b00764 ↗
21. 10.1021/acs.chemmater.8b0335210.1021/acs.chemmater.8b03352 ↗
22. 10.1002/adfm.20190516310.1002/adfm.201905163 ↗
23. 10.1002/adfm.20190360710.1002/adfm.201903607 ↗
24. 10.1021/acsami.9b0510110.1021/acsami.9b05101 ↗
25. 10.1021/acsenergylett.7b0121710.1021/acsenergylett.7b01217 ↗
26. 10.1002/aenm.20170350610.1002/aenm.201703506 ↗
27. 10.1038/s41566-019-0398-210.1038/s41566-019-0398-2 ↗
28. 10.1039/c7tc02477k10.1039/c7tc02477k ↗
29. 10.1002/adfm.20180734510.1002/adfm.201807345 ↗
30. 10.1021/acs.nanolett.5b0495910.1021/acs.nanolett.5b04959 ↗
31. 10.1021/acsami.9b1018610.1021/acsami.9b10186 ↗
32. 10.1016/j.joule.2018.06.01310.1016/j.joule.2018.06.013 ↗
33. 10.1039/c8nr06311g10.1039/c8nr06311g ↗
34. 10.1002/adom.20180124510.1002/adom.201801245 ↗
35. 10.1002/adfm.20180418710.1002/adfm.201804187 ↗
36. 10.1021/acs.jpclett.7b0130210.1021/acs.jpclett.7b01302 ↗
37. 10.1016/j.orgel.2019.01.03010.1016/j.orgel.2019.01.030 ↗
38. 10.1039/c7ta09646a10.1039/c7ta09646a ↗