journal article·2019-02-01Open access

Ultrafast nonlinear transparency driven at a telecom wavelength in an organic semiconductor system

Joong-Mok Park, Di Cheng, Aaron Patz, Liang Luo, Zhaoyu Liu, Fadzai Fungura, Ruth Shinar, Kai-Ming Ho, Joseph Shinar, Jigang Wang

AIP Advances· Volume 9· Issue 2

Abstract

Ultrafast laser-induced transparency is demonstrated using femtosecond (fs) pump-probe experiments in the organic P3HT:PCBM (donor:acceptor) blend structure. For above band gap pumping, ultrafast transient signals strongly depend on the probe photon energy. Most intriguingly, for below band gap pumping at 0.95 eV, or 1.3 µm at a telecom wavelength, a huge transmission increase up to 30% only during the laser pulse ∼100 fs is observed as a pump-driven, quasi-instantaneous suppression of absorption for the high photon-energy energy probe beam. We attribute the observed laser-driven transparency to dynamic Franz-Keldysh effect, at least one order of magnitude stronger compared to the multiphoton nonlinearities. Our results may be used for development of low-cost, beyond 100 Gbit/s optical switching devices.
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Research context

OpenAlex topics: Photonic and Optical Devices · Mechanical and Optical Resonators · Nonlinear Optical Materials Studies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Ames Laboratory - USDOE 1 , Ames, Iowa 50011, USA

Department of Physics and Astronomy, Iowa State University 2 , Ames, Iowa 50011, USA

Microelectronics Research Center 3 , Ames, Iowa 50011, USA

Funding

Department of Energy of USA

References (52)

Show source-provided references
1. A review of ultrafast optics and optoelectronics10.1088/1464-4258/5/1/201 ↗
2. All-optical signal processing for terabit/second optical transmission10.1109/2944.902190 ↗
3. Ultrahigh-speed OTDM-transmission technology10.1109/jlt.2006.885784 ↗
4. Technologies for optical systems beyond 100G10.1016/j.yofte.2011.06.007 ↗
5. Optical integration and multi-carrier solutions for 100G and beyond10.1016/j.yofte.2011.07.005 ↗
6. Organic photonics for communications10.1038/nphoton.2010.160 ↗
7. Subnanosecond Pockels cell switching using avalanche transistors10.1063/1.2194472 ↗
8. Ultrafast optical control using the Kerr nonlinearity in hydrogenated amorphous silicon microcylindrical resonators10.1038/srep02885 ↗
9. Femtosecond laser excitation of the semiconductor-metal phase transition in VO210.1063/1.112974 ↗
10. Fast all-optical switching using ion-implanted silicon photonic crystal nanocavities10.1063/1.2431767 ↗
11. Sub-femtojoule all-optical switching using a photonic-crystal nanocavity10.1038/nphoton.2010.89 ↗
12. Ultrafast all-optical switching in semiconductor nonlinear directional couplers at half the band gap10.1063/1.108200 ↗
13. Excitonic dynamical Franz-Keldysh effect10.1103/physrevlett.81.457 ↗
14. Quantum interface and control of the dynamic Franz-Keldysh effect: Generation and detection of terahertz space-charge fields10.1063/1.4811709 ↗
15. Ultrafast electroabsorption at the transition between classical and quantum response10.1103/physrevlett.85.3293 ↗
16. Laser-induced above-band-gap transparency in GaAs10.1103/physrevlett.93.157401 ↗
17. Recent progress in polymer solar cells: Manipulation of polymer:Fullerene morphology and the formation of efficient inverted polymer solar cells10.1002/adma.200802854 ↗
18. High-efficiency solution processable polymer photovoltaic cells by self-organization of polymer blends10.1038/nmat1500 ↗
19. Roles of donor and acceptor nanodomains in 6% efficient thermally annealed polymer photovoltaics10.1063/1.2730756 ↗
20. Coherent ultrafast charge transfer in an organic photovoltaic blend10.1126/science.1249771 ↗
21. Effect of morphology on ultrafast free carrier generation in polythiophene:Fullerene organic solar cells10.1021/ja105260d ↗
22. Nonequilibrium charge dynamics in organic solar cells10.1002/aenm.201301743 ↗
23. Ultrafast energy transfer in ultrathin organic donor/acceptor blend10.1038/srep02073 ↗
24. Interplay between side chain pattern, polymer aggregation, and charge carrier dynamics in PBDTTPD:PCBM bulk-heterojunction solar cells10.1002/aenm.201401778 ↗
25. The effect of solvent additives on morphology and excited-state dynamics in PCPDTBT:PCBM photovoltaic blends10.1021/ja303154g ↗
26. Hot exciton dissociation in polymer solar cells10.1038/nmat3502 ↗
27. Influence of blend composition on ultrafast charge generation and recombination dynamics in low band gap polymer-based organic photovoltaics10.1021/jp302787u ↗
28. The role of driving energy and delocalized states for charge separation in organic semiconductors10.1126/science.1217745 ↗
29. Charge formation, recombination, and sweep-out dynamics in organic solar cells10.1002/adfm.201101632 ↗
30. Ultrafast optical and magneto-optical studies of III-V ferromagnetic semiconductors10.1080/09500340408231836 ↗
31. Theory of carrier dynamics and time-resolved reflectivity in InxMn1–xAs/GaSb heterostructures10.1103/physrevb.72.245302 ↗
32. Ultrafast observation of critical nematic fluctuations and giant magnetoelastic coupling in iron pnictides10.1038/ncomms4229 ↗
33. Design rules for donors in bulk-heterojunction solar cells - towards 10% energy-conversion efficiency10.1002/adma.200501717 ↗
35. High performance polymer solar cells with as-prepared zirconium acetylacetonate film as cathode buffer layer10.1038/srep04691 ↗
36. Electronic structure and transition energies in polymer−fullerene bulk heterojunctions10.1021/jp507097h ↗
37. Optical absorption study of P3HT:PCBM blend photo-oxidation for bulk heterojunction solar cells10.1016/j.solener.2016.05.009 ↗
38. Reversible modulation and ultrafast dynamics of terahertz resonances in strongly photoexcited metamaterials10.1103/physrevb.86.125110 ↗
39. Terahertz light-quantum-tuning of a metastable emergent phase hidden by superconductivity10.1038/s41563-018-0096-3 ↗
40. Ultrafast softening in InMnAs10.1016/j.physe.2003.08.048 ↗
41. Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite10.1038/ncomms15565 ↗
42. Spatial-temporal spectroscopy characterizations and electronic structure of methyl-ammonium perovskites
43. The path to ubiquitous and low-cost organic electronic appliances on plastic10.1038/nature02498 ↗
44. Flexible blade-coated multicolor polymer light-emitting diodes for optoelectronic sensors10.1002/adma.201606206 ↗
45. Wearable organic optoelectronic sensors for medicine10.1002/adma.201403560 ↗
46. Long-term stabilization of organic solar cells using UV absorbers10.1088/0022-3727/49/12/125604 ↗
47. Current status of outdoor lifetime testing of organic photovoltaics10.1002/advs.201800434 ↗
48. Highly efficient, large area, roll coated flexible and rigid OPV modules with geometric fill factors up to 98.5% processed with commercially available materials10.1039/c5ee03315b ↗
49. A series connection architecture for large-area organic photovoltaic modules with a 7.5% module efficiency10.1038/ncomms10279 ↗
50. Fabrication of bulk heterojunction plastic solar cells by screen printing10.1063/1.1413501 ↗
51. Attosecond dynamical Franz-Keldysh effect in polycrystalline diamond10.1126/science.aag1268 ↗
52. Ultrafast terahertz probes of interacting dark excitons in chirality-specific semiconducting single-walled carbon nanotubes10.1103/physrevlett.114.107402 ↗