journal article·2021-08

Enhanced performance by inducing defect dipoles in lead based relaxor ferroelectric PHT-based ceramics

Weiqian Song, Yangxi Yan, Maolin Zhang, Dongyan Zhang, Li Jin, Zhimin Li

Ceramics International· Volume 47· Issue 16
Publisher page

Abstract

Abstract Mn-doped 0.49 Pb(Ni1/3Nb2/3)O3-0.51 Pb(Hf0.3Ti0.7)O3 (abbreviated PNN-PHT) ceramics were prepared by solid-phase reaction method. The influence of defect dipoles on various properties was systematically studied. Results showed that Mn doping significantly improved mechanical quality factor Qm of PNN-PHT ceramics and greatly reduced dielectric loss, while Curie temperature Tc was also slightly increased. After 105 electric field cycles, Mn doped PNN-PHT ceramic showed excellent fatigue property. Based on ferroelectric and dielectric properties of samples, the reason for defect dipole and internal mechanism of its influence on piezoelectric properties were elucidated. Finally, novel ceramic 0.75 mol% Mn-doped PNN-PHT with excellent performance was obtained (d33~750 pC/N, kp~0.55, Qm~384 and tanδ~0.59%). Therefore, results of this work suggest that these ceramics may be potential candidates for piezoelectric actuators and high-power devices.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Ferroelectric and Piezoelectric Materials · Dielectric materials and actuators · Acoustic Wave Resonator Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (60)

Show source-provided references
1. Piezoelectric materials and their applications10.4028/www.scientific.net/KEM.122-124.71 ↗
2. Piezoelectric activity in perovskite ferroelectric crystals10.1109/TUFFC.2014.006660 ↗
3. Electromechanical properties of Mn-doped Pb(In1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 piezoelectric ceramics10.1016/j.ceramint.2016.06.175 ↗
4. What can be expected from lead-free piezoelectric materials10.1142/S1793604710000919 ↗
5. Lead-free piezoelectric ceramics: alternatives for PZT10.1007/s10832-007-9047-0 ↗
6. Effect of MnO2 on the microstructure and electrical properties of 0.83Pb(Zr0.5Ti0.5)O3-0.11Pb(Zn1/3Nb2/3)O3-0.06Pb(Ni1/3Nb2/3)O3 piezoelectric ceramics10.1016/j.ceramint.2019.08.246 ↗
7. Effect of rare-earth addition on morphotropic phase boundary and relaxation behavior of the PNN-PZT ceramics
8. Ferroelectric and electromechanical performance of diverse engineered states of Mn-doped 0.75Pb(Mg1/3Nb2/3)O3-0.25PbTiO3 ceramics10.1016/j.ceramint.2021.03.165 ↗
9. Crystal structure and piezoelectric characteristics of various phases near the triple-point composition in PZ-PT-PNN system10.1016/j.jeurceramsoc.2019.12.063 ↗
10. Raman spectra and structural stability in B-site manganese doped (Bi0.5Na0.5)0.925Ba0.075TiO3 relaxor ferroelectric ceramics10.1016/j.jeurceramsoc.2015.05.002 ↗
11. Defect engineering in lead zirconate titanate ferroelectric ceramic for enhanced electromechanical transducer efficiency
12. Investigation of switching behavior of acceptor-doped ferroelectric ceramics10.1016/j.actamat.2019.03.033 ↗
13. Ultrahigh electro-strain in acceptor-doped KNN lead-free piezoelectric ceramics via defect engineering10.1016/j.actamat.2020.08.073 ↗
14. Effect of MnO2 doping on piezoelectric, dielectric and ferroelectric properties of PNN-PZT ceramics10.1016/j.ceramint.2015.05.094 ↗
15. Nanodomains in Fe3+-doped lead zirconate titanate ceramics at the morphotropic phase boundary do not correlate with high properties10.1063/1.3173198 ↗
16. Domain wall contributions in Pb(Zr, Ti)O3 ceramics at morphotropic phase boundary: a study of dielectric dispersion10.1063/1.3455328 ↗
17. Lattice dynamics and dielectric response of undoped, soft and hard PbZr0.42Ti0.58O310.1080/01411594.2010.509601 ↗
18. Effect of annealing on defect and electrical properties of Mn doped Pb(Mg1/3Nb2/3)O3-0.28PbTiO3 single crystals10.1016/j.jcrysgro.2010.10.187 ↗
19. Orientation dependence of piezoelectric properties and mechanical quality factors of 0.27Pb(In1/2Nb1/2)O3-0.46Pb(Mg1/3Nb2/3)O3-0.27PbTiO3: Mn single crystals10.1063/1.4821030 ↗
20. Tuning the functional properties of PMN-PT single crystals via doping and thermoelectrical treatments10.1063/1.4847975 ↗
21. Improved thermal stability of [001]c poled 0.24Pb(In1/2Nb1/2)O3-0.47Pb(Mg1/3Nb2/3)O3-0.29PbTiO3 single crystal with manganese doping10.1016/j.jallcom.2014.02.174 ↗
22. Impacts of acceptor doping on the piezoelectric properties and domain structure in NBT-based lead-free ceramics10.1016/j.jeurceramsoc.2017.04.047 ↗
23. Enhanced piezoelectric properties of 0.49Pb(Ni, Nb)O3-0.51Pb(Hf, Ti)O3 ceramics by ion pair doping
24. Identification and effect of secondary phase in MnO2-doped 0.8Pb(Zr0.52Ti0.48)O3-0.2Pb(Zn1/3Nb2/3)O3 piezoelectric ceramics10.1111/j.1551-2916.2011.04629.x ↗
25. Effects of MnO2 additive on the properties of PbZrO3-PbTiO3-PbCu1/4Nb3/4O3 ferroelectric ceramic system10.1016/S0955-2219(00)00216-8 ↗
26. Phase diagram and properties of Pb(In1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 polycrystalline ceramics10.1016/j.jeurceramsoc.2011.08.025 ↗
27. Fabrication and characterisation of ferroelectric perovskite lead indium niobate10.1080/00150198508008960 ↗
28. Effects of Mn doping on the structure and electrical properties of high-temperature BiScO3-PbTiO3-Pb(Zn1/3Nb2/3)O3 piezoelectric ceramics10.1016/j.materresbull.2011.03.034 ↗
29. Impacts of acceptor doping on the piezoelectric properties and domain structure in NBT-based lead-free ceramics10.1016/j.jeurceramsoc.2017.04.047 ↗
30. Fabrication and properties of nonreducible lead-free piezoelectric Mn-doped (Ba, Ca)TiO3 ceramics10.1016/j.ceramint.2017.05.291 ↗
31. Effects of addition of MnO on piezoelectric properties of lead zirconate titanate10.1023/A:1004717702149 ↗
32. Double hysteresis loop in Cu-doped K0.5Na0.5NbO3 lead-free piezoelectric ceramics10.1063/1.2746087 ↗
33. Of Fe-doped potassium sodium niobate tantalate lead-free ceramics10.1111/j.1551-2916.2011.04390.x ↗
34. Defects and charge transport in Mn-doped K0.5Na0.5NbO3 ceramics10.1039/C5CP02883C ↗
35. Defect structure in aliovalently-doped and isovalently-substituted PbTiO3 nano-powders10.1088/0953-8984/22/34/345901 ↗
36. Studying the roles of Cu and Sb in K0.48Na0.52NbO3 lead-free piezoelectric ceramics10.1016/j.jallcom.2015.03.223 ↗
37. Time dependence of the mechanical quality factor in "hard" lead zirconate titanate ceramics: development of an internal dipolar field and high power origin10.1143/JJAP.45.9119 ↗
38. Large strain induced by the alignment of defect dipoles in (Bi3+, Fe3+) co-doped Pb(Zr, Ti)O3 ceramics10.1016/j.scriptamat.2017.08.013 ↗
39. Decoding the fingerprint of ferroelectric loops: comprehension of the material properties and structures10.1111/jace.12773 ↗
40. Enhanced piezoelectric properties by reducing leakage current in Co modified 0.7BiFeO3-0.3BaTiO3 ceramics10.1016/j.ceramint.2018.02.095 ↗
41. Poling of hard ferroelectric PZT ceramics10.1016/j.jeurceramsoc.2007.11.023 ↗
42. Domain wall clamping in ferroelectrics by orientation of defects10.1063/1.352948 ↗
43. Effects of Mn doping on multiferroic and magnetocapacitive properties of 0.33Ba0.70Ca0.30TiO3-0.67BiFeO3 diphasic ceramics10.1016/j.jallcom.2013.11.029 ↗
44. Textured Mn-doped PIN-PMN-PT ceramics: harnessing intrinsic piezoelectricity for high-power transducer applications10.1016/j.jeurceramsoc.2020.07.071 ↗
45. Low-temperature sintering and electrical properties of PGO-doped PNN-PZT ceramics
46. Processing and electrical properties of 0.5Pb(Yb1/2Nb1/2)O3-0.5PbTiO3 ceramics10.1023/A:1024080008850 ↗
47. The high piezoelectric properties and high temperature stability in Mn doped Pb(Mg0.5W0.5)O3-Pb(Zr, Ti)O3 ceramics10.1016/j.ceramint.2018.12.144 ↗
48. Enhancing piezoelectric properties of Ba0.88Ca0.12Zr0.12Ti0.88O3 lead-free ceramics by doping Co ions-Science Direct10.1016/j.ceramint.2020.09.167 ↗
49. Large electro-strain with excellent fatigue resistance of lead-free (Bi0.5Na0.5)0.94Ba0.06Ti1-x(Y0.5Nb0.5)xO3 perovskite ceramics
50. The effect of uniaxial pressure, temperature and electric field on the internal bias field in the lead-based piezoelectric ceramics10.1016/j.matlet.2015.10.156 ↗
51. Bipolar and unipolar fatigue property in Bi0.5Na0.5TiO3-Bi0.5K0.5TiO3-SrTiO3 lead-free piezoelectric ceramics10.1016/j.physb.2019.411716 ↗
52. Effects of ZnO/Li2O codoping on microstructure and piezoelectric properties of low temperature sintered PMN-PNN-PZT ceramics10.1016/j.ceramint.2009.03.012 ↗
53. Characterization of hard piezoelectric lead-free ceramics10.1109/TUFFC.2009.1215 ↗
54. Dielectric, ferroelectric and piezoelectric properties of MnO2-doped Pb(Yb1/2Nb1/2)O3-Pb(Zr,Ti)O3 ceramics10.1016/j.ceramint.2018.02.042 ↗
55. Low temperature sintering of Pb(Ni, Nb)O3-Pb(Hf, Ti)O3 piezoceramics with Fe2O3 and Bi2O3 addition10.1016/j.ceramint.2018.08.321 ↗
56. Improving piezoelectric properties of Pb(Ni,Nb)O3-Pb(Hf,Ti)O3 ceramics by LiF addition10.1016/j.ceramint.2017.12.094 ↗
57. Effect of MnO2 addition on the microstructure and electrical properties of Pb(Zn1/3Nb2/3)0.20(Zr0.50Ti0.50)0.80O3 ceramics10.1111/j.1551-2916.2004.00847.x ↗
58. Size effects in Fe3+-doped PbTiO3 nanocrystals-formation and orientation of (Fe, Ti-Vo) defect-dipoles10.1016/j.jeurceramsoc.2009.04.034 ↗
59. Enhanced piezoelectric properties and constricted hysteresis behaviour in PZT ceramics induced by Li+-Al3+ ionic pairs10.1039/C6RA00152A ↗
60. Piezoelectric properties in the perovskite BiScO3-PbTiO3-(Ba, Sr)TiO3 ternary system10.1143/JJAP.42.5181 ↗