journal article·2017-07

Effects of Mn doping on dielectric properties and energy-storage performance of Na0.5Bi0.5TiO3 thick films

Jiaheng Wang, Ningning Sun, Yong Li, Qiwei Zhang, Xihong Hao, Xiujian Chou

Ceramics International· Volume 43· Issue 10
Publisher page

Abstract

Abstract Lead-free Na 0.5 Bi 0.5 Ti 1−x Mn x O 3 (NBTMn x , x=0, 0.01, 0.03 and 0.05) ferroelectric thick films have been fabricated on LaNiO 3 /Si(100) substrate by using a polyvinylpyrrolidone-modified sol-gel method and the effects of Mn content on their microstructure, dielectric properties and energy-storage performance were investigated. Compared with the pure Na 0.5 Bi 0.5 TiO 3 (NBT) thick films, NBTMn x thick films exhibited a large enhancement in dielectric properties and energy-storage performance. Particularly, a giant recoverable energy-storage density ( W ) of 30.2 J/cm 3 and the corresponding efficiency ( η ) of 47.7% were obtained in NBTMn 0.01 thick film at 2310 kV/cm. Moreover, the NBTMn 0.01 thick film displayed good energy-storage stability over a large temperature range at different frequency.
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Research context

OpenAlex topics: Ferroelectric and Piezoelectric Materials · Dielectric materials and actuators · Multiferroics and related materials

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References (37)

Show source-provided references
1. A lead-free and high-energy density ceramic for energy storage applications10.1111/jace.12508 ↗
2. Bi0.5Na0.5TiO3–BaTiO3 based thick-film capacitors for high-temperature applications10.1016/j.jeurceramsoc.2013.07.020 ↗
3. Effect of MgO–CaO–Al2O3–SiO2 glass additive on dielectric properties of Ba0.95Sr0.05Zr0.2Ti0.8O3 ceramics10.1016/j.jallcom.2012.12.164 ↗
4. Preparation and energy-storage performance of PLZT antiferroelectric thick films via sol–gel method10.1016/j.ceramint.2012.10.124 ↗
5. High energy-storage performance and dielectric properties of antiferroelectric (Pb0.97La0.02)(Zr0.5Sn0.5−xTix)O3 ceramic10.1016/j.jallcom.2015.09.167 ↗
6. Composition-dependent dielectric and energy-storage properties of (Pb,La)(Zr,Sn,Ti)O3 antiferroelectric thick films10.1063/1.4802794 ↗
7. Large energy storage density and high thermal stability in a highly textured (111)-oriented Pb0.8Ba0.2ZrO3 relaxor thin film with the coexistence of antiferroelectric and ferroelectric phases10.1021/acsami.5b02790 ↗
8. Antarctic-wide array of high-resolution ice core records reveals pervasive lead pollution began in 1889 and persists today10.1038/srep05848 ↗
9. A review of soil heavy metal pollution from mines in China: pollution and health risk assessment10.1016/j.scitotenv.2013.08.090 ↗
10. New ferroelectrics with complex compounds
11. Dielectric and impedance spectroscopy of zirconium (Na0.5Bi0.5)TiO3 ceramics10.1016/j.ceramint.2012.12.087 ↗
12. Giant strain in lead-free (Bi0.5Na0.5)TiO3-based single crystals10.1063/1.2920767 ↗
13. Large piezoresponse of Na0.5Bi0.5TiO3–K0.5Bi0.5TiO3 thin films prepared via water-based sol–gel method10.1016/j.ceramint.2015.03.232 ↗
14. Electrical properties of (1–x)(Bi0.5Na0.5)TiO3-xBaTiO3 synthesized by emulsion method10.1016/j.ceramint.2005.10.022 ↗
15. Sonia, Dielectric and ferroelectric study of KNN modified NBT ceramics synthesized by microwave processing technique10.1016/j.ceramint.2012.10.005 ↗
16. Microstructure, ferroelectric and dielectric properties of sandwich structure for Na0.5Bi0.5TiO3 thin film modified with aliovalent substitution10.1016/j.ceramint.2015.10.160 ↗
17. Effect of Fe doping on the crystallization and electrical properties of Na0.5Bi0.5TiO3 thin film10.1016/j.ceramint.2014.10.066 ↗
18. Dielectric properties and energy-storage performance of (Na0.5Bi0.5)TiO3–SrTiO3 thick films derived from polyvinylpyrrolidone-modified chemical solution10.1016/j.jallcom.2015.03.133 ↗
19. Microstructure and energy-storage performance of PbO-B2O3-SiO2-ZnO glass added (Pb0.97La0.02)(Zr0.97Ti0.03)O3 antiferroelectric thick films10.1016/j.materresbull.2012.10.005 ↗
20. Dielectric properties and energy-storage performance of (Na0.5Bi0.5)TiO3 thick films10.1016/j.jallcom.2014.02.137 ↗
21. Preparation of highly (100)-oriented metallic LaNiO3 films on Si substrates by a modified metalorganic decomposition technique10.1016/S0169-4332(00)00537-7 ↗
22. Structure and electrical properties of (Na0.5Bi0.5)TiO3 ferroelectric thick films derived from a polymer modified sol-gel method10.1109/TUFFC.2011.2054 ↗
23. Effect of Mn doping on microstructure and electrical properties of the (Na0.85K0.15)0.5Bi0.5TiO3 thin films prepared by sol–gel method10.1111/j.1551-2916.2011.04576.x ↗
24. Ferroelectric PLZT thick films grown by poly (1-vinylpyrrolidone-co-vinyl acetate)(PVP/VA)-modified sol–gel process10.1016/j.materresbull.2015.11.049 ↗
25. Microstructure and electrical properties mediated by defects in Na0.5Bi0.5Ti0.98Mn0.02O3 thin film under different annealing atmospheres10.1016/j.jeurceramsoc.2015.10.015 ↗
26. The microstructure, ferroelectric and dielectric behaviors of Na0.5Bi0.5(Ti,Fe)O3 thin films synthesized by chemical solution deposition: effect of precursor solution concentration10.1016/j.ceramint.2016.10.173 ↗
27. Temperature and frequency dependence of dielectric properties of (Pb,La)(Zr,Sn,Ti)O3 antiferroelectric thin films on LaNiO3 bottom electrode with different sheet resistance10.1088/0022-3727/41/16/165403 ↗
28. Orientation-dependent dielectric properties of Ba(Sn0.15Ti0.85)O3 thin films prepared by sol–gel method10.1016/j.jpcs.2009.07.007 ↗
29. Dielectric breakdown in high-ε films for ULSI DRAMs10.1080/10584589308216715 ↗
30. Defect dipole induced large recoverable strain and high energy-storage density in lead-free Na0.5Bi0.5TiO3-based systems10.1063/1.4950974 ↗
31. Relaxor behavior and energy storage performance of ferroelectric PLZT thin films with different Zr/Ti ratios10.1016/j.ceramint.2013.05.139 ↗
32. Enhanced energy-storage properties of 0.89Bi0.5Na0.5TiO3-0.06BiTiO3-0.05K0.5Na0.5NbO3 lead-free anti-ferroelectric ceramics by two-step sintering method10.1016/j.matlet.2013.09.103 ↗
33. Enhanced energy-storage properties of (1-x)[(1-y)(Bi0.5Na0.5)TiO3-y(Bi0.5K0.5)TiO3]-x(K0.5Na0.5)NbO3 lead-free ceramics10.1016/j.ssc.2014.12.004 ↗
34. High energy-storage properties of [(Bi1/2Na1/2)0.94Ba0.06] La(1-x)ZrxTiO3 lead-free anti-ferroelectric ceramics10.1016/j.ceramint.2013.08.099 ↗
35. High energy storage properties and dielectric behavior of (Bi0.5Na0.5)0.94Ba0.06Ti1−x(Al0.5Nb0.5)xO3 lead-free ferroelectric ceramics10.1016/j.ceramint.2015.10.014 ↗
36. Enhanced energy-storage performance of 0.94NBT-0.06BT thin films induced by a Pb0.8La0.1Ca0.1Ti0.975O3 seed layer10.1016/j.ceramint.2016.06.110 ↗
37. High-energy-storage density capacitors of Bi(Ni1/2Ti1/2)O3-PbTiO3 thin films with good temperature stability10.1111/jace.12443 ↗