journal article·2017-05

Photocatalysis of composite film PDMS-PMN-PT@TiO2 greatly improved via spatial electric field

Baoying Dai, Ling Zhang, Hengming Huang, Chunhua Lu, Jiahui Kou, Zhongzi Xu

Publisher page

Abstract

Efficient charge separation is quite significant to obtain high photocatalytic performance. In this work, piezoelectric-based composite photocatalyst film PDMS-PMN-PT@TiO2 possessing high recoverability was prepared. The spatial electric field of PMN-PT was introduced into photocatalyst system by ultrasonic wave vibration to accelerate charge separation. Compared with magnetic stirring, ultrasonic wave vibration greatly improved the photocatalytic degradation efficiency of rhodamine B (RhB) over PDMS-PMN-PT@TiO2 film by about 55%. A possible improvement mechanism that spatial electric field promotes charge separation was presented herein. The piezoelectric potential output demonstrated the piezoelectricity of composite film. The durability experiments of PDMS-PMN-PT@TiO2 film indicated its great stability over several runs.
Source: openaire · Quality: candidate unverified · Source record ↗

Research context

OpenAlex topics: Advanced Sensor and Energy Harvesting Materials · Advanced Photocatalysis Techniques · Gas Sensing Nanomaterials and Sensors

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

References (25)

Show source-provided references
1. Research progress of perovskite materials in photocatalysis- and photovoltaics-related energy conversion and environmental treatment10.1039/C5CS00113G ↗
2. Au-nanoparticle-loaded graphitic carbon nitride nanosheets: green photocatalytic synthesis and application toward the degradation of organic pollutants10.1021/am401802r ↗
3. Reusable electrospun mesoporous ZnO nanofiber mats for photocatalytic degradation of polycyclic aromatic hydrocarbon dyes in wastewater10.1016/j.jcis.2012.12.006 ↗
4. Magnetic titanium dioxide based nanomaterials: synthesis, characteristics, and photocatalytic application in pollutant degradation10.1039/C5TA03215F ↗
5. Enhancement of visible photocatalytic activity via Ag@C3N4 core-shell plasmonic composite10.1016/j.apcatb.2013.08.007 ↗
6. Aluminum plasmonics for enhanced visible light absorption and high efficiency water splitting in core-multishell nanowire photoelectrodes with ultrathin hematite shells10.1021/nl501541s ↗
7. Charge separation and catalytic activity of Ag@TiO2 core-shell composite clusters under UV-irradiation10.1021/ja042925a ↗
8. Heterostructured visible-light-active photocatalyst of chromia-nanoparticle-layered titanate10.1002/adfm.200600022 ↗
9. Piezotronic effect enhanced photocatalysis in strained anisotropic ZnO/TiO2 nanoplateletsvia thermal stress10.1021/acsnano.5b07678 ↗
10. Piezo-potential enhanced photocatalytic degradation of organic dye using ZnO nanowires10.1016/j.nanoen.2015.02.029 ↗
11. Enhanced ferroelectric-nanocrystal-based hybrid photocatalysis by ultrasonic-wave-generated piezophototronic effect10.1021/nl504630j ↗
12. Flexible piezoelectric PMN-PT nanowire-based nanocomposite and device10.1021/nl400169t ↗
13. Fabrication and piezoelectric property of PMN-PT nanofibers10.1016/j.nanoen.2012.03.011 ↗
14. Numerical study of acoustophoretic motion of particles in a PDMS microchannel driven by surface acoustic waves10.1039/C5LC00231A ↗
15. Highly flexible piezoelectric 0-3 PZT-PDMS composites with high filler content10.1016/j.compscitech.2013.11.027 ↗
16. Enhanced photoactivity with nanocluster-grafted titanium dioxide photocatalysts10.1021/nn502247x ↗
17. Controllable synthesis of mesoporous TiO2 hollow shells: toward an efficient photocatalyst10.1002/adfm.201300255 ↗
18. Superhydrophilic TiO2 thin film by nanometer scale surface roughness and dangling bonds10.1016/j.apsusc.2015.12.108 ↗
19. Hydrothermal synthesis and photocatalytic activity of nanocrystalline TiO2 powders in ethanol-water mixed solutions10.1016/j.molcata.2007.05.009 ↗
20. Shi · 2008
21. Electric field enhanced photocatalytic properties of TiO2 nanoparticles immobilized in porous silicon template10.1016/j.solidstatesciences.2011.05.010 ↗
22. Study on electromechanical characterization of piezoelectric polymer PVDF in low-frequency band10.1007/s10854-014-2225-3 ↗
23. PMN-PT nanowires with a very high piezoelectric constant10.1021/nl204334x ↗
24. Titanium oxide-reduced graphene oxide-silver composite layers synthesized by laser technique: wetting and electrical properties10.1016/j.ceramint.2016.07.140 ↗
25. Fine-tuning of surface properties of dual-size TiO2 nanoparticle coatings10.1016/j.surfcoat.2016.07.059 ↗