Tunable wrinkle patterns in Moiré pattern of interlayer-bonding strained bilayer graphene

Moiré patterns are important structures in two-dimensional (2D) materials, showcasing unique electronic correlated states, which have garnered considerable research interests in recent years. However, current researches on moiré patterns primarily focus on honeycomb patterns induced by lattice mismatches at 2D material hetero-interfaces. In this work, we have demonstrated the ability to generate diverse and tunable wrinkle patterns in interlayer bonding strained bilayer graphene (IB-SBG) through a “stretch-crosslink-release” strategy, facilitated by the interlayer bonding that provides effective in-plane load transfer and interlayer constraint. Three energetically favorable wrinkle patterns are identified, including herringbone, irregular hexagon and honeycomb patterns. In general, wrinkle patterns are determined by two parameters, i.e., pre-strain and the portion of interface with interlayer bonding, and the phase diagram of wrinkle patterns corresponding to the two parameters is provided. Furthermore, strain engineering can be employed in IB-SBG to generate a series of new patterns by precisely adjusting the biaxial strain applied to IB-SBG. The present strategy to achieve tunable wrinkle patterns holds the potential to open new avenues for novel electronic applications based on bilayer graphene systems.