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This cover illustrates the molecular engineering of donor–acceptor (D‐A) frameworks, where fine tuning of the central core and end groups enables wide‐spectrum photodetection from ultraviolet to near‐infrared. By applying such tailored organic semiconductors to organic field‐effect transistor arrays and integrating them into neuromorphic network architectures, the device achieves bio‐inspired vision with spectral adaptability. The design highlights a synergistic pathway from precise molecular design to intelligent, wide‐spectrum perception for next‐generation optoelectronic systems. image