journal article·2022-10-01Open access

Exciton optics, dynamics, and transport in atomically thin semiconductors

Raul Perea-Causin, Daniel Erkensten, Jamie M. Fitzgerald, Joshua J. P. Thompson, Roberto Rosati, Samuel Brem, Ermin Malic

APL Materials· Volume 10· Issue 10

Abstract

Atomically thin semiconductors such as transition metal dichalcogenide (TMD) monolayers exhibit a very strong Coulomb interaction, giving rise to a rich exciton landscape. This makes these materials highly attractive for efficient and tunable optoelectronic devices. In this Research Update, we review the recent progress in the understanding of exciton optics, dynamics, and transport, which crucially govern the operation of TMD-based devices. We highlight the impact of hexagonal boron nitride-encapsulation, which reveals a plethora of many-particle states in optical spectra, and we outline the most novel breakthroughs in the field of exciton-polaritonics. Moreover, we underline the direct observation of exciton formation and thermalization in TMD monolayers and heterostructures in recent time-resolved, angle-resolved photoemission spectroscopy studies. We also show the impact of exciton density, strain, and dielectric environment on exciton diffusion and funneling. Finally, we put forward relevant research directions in the field of atomically thin semiconductors for the near future.
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Research context

OpenAlex topics: 2D Materials and Applications · Perovskite Materials and Applications · Strong Light-Matter Interactions

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, Chalmers University of Technology 1 , 412 96 Gothenburg, Sweden

Department of Physics, Philipps-Universität Marburg 2 , 35032 Marburg, Germany

Funding

Deutsche Forschungsgemeinschaft · Graphene Flagship

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