journal article·2021-10-01Open access

Roadmap on organic–inorganic hybrid perovskite semiconductors and devices

Lukas Schmidt-Mende, Vladimir Dyakonov, Selina Olthof, Feray Ünlü, Khan Moritz Trong Lê, Sanjay Mathur, Andrei D. Karabanov, Doru C. Lupascu, Laura M. Herz, Alexander Hinderhofer, Frank Schreiber, Alexey Chernikov, David A. Egger, Oleksandra Shargaieva, Caterina Cocchi, Eva Unger, Michael Saliba, Mahdi Malekshahi Byranvand, Martin Kroll, Frederik Nehm, Karl Leo, Alex Redinger, Julian Höcker, Thomas Kirchartz, Jonathan Warby, Emilio Gutierrez-Partida, Dieter Neher, Martin Stolterfoht, Uli Würfel, Moritz Unmüssig, Jan Herterich, Clemens Baretzky, John Mohanraj, Mukundan Thelakkat, Clément Maheu, Wolfram Jaegermann, Thomas Mayer, Janek Rieger, Thomas Fauster, Daniel Niesner, Fengjiu Yang, Steve Albrecht, Thomas Riedl, Azhar Fakharuddin, Maria Vasilopoulou, Yana Vaynzof, Davide Moia, Joachim Maier, Marius Franckevičius, Vidmantas Gulbinas, Ross A. Kerner, Lianfeng Zhao, Barry P. Rand, Nadja Glück, Thomas Bein, Fabio Matteocci, Luigi Angelo Castriotta, Aldo Di Carlo, Matthias Scheffler, Claudia Draxl

APL Materials· Volume 9· Issue 10

Abstract

Metal halide perovskites are the first solution processed semiconductors that can compete in their functionality with conventional semiconductors, such as silicon. Over the past several years, perovskite semiconductors have reported breakthroughs in various optoelectronic devices, such as solar cells, photodetectors, light emitting and memory devices, and so on. Until now, perovskite semiconductors face challenges regarding their stability, reproducibility, and toxicity. In this Roadmap, we combine the expertise of chemistry, physics, and device engineering from leading experts in the perovskite research community to focus on the fundamental material properties, the fabrication methods, characterization and photophysical properties, perovskite devices, and current challenges in this field. We develop a comprehensive overview of the current state-of-the-art and offer readers an informed perspective of where this field is heading and what challenges we have to overcome to get to successful commercialization.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Quantum Dots Synthesis And Properties · Conducting polymers and applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics, University of Konstanz 1 , Universitaetsstr. 10, 78457 Konstanz, Germany

Experimental Physics VI, University of Würzburg 2 , Am Hubland, 97074 Würzburg, Germany

Department of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, Germany

Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen 4 , 45141 Essen, Germany

Clarendon Laboratory, Department of Physics, University of Oxford 5 , Parks Road, Oxford OX1 3PU, United Kingdom

TUM Institute for Advanced Study 6 , 85748 Garching bei München, Germany

Institute of Applied Physics, University of Tübingen 7 , Auf der Morgenstelle 10, 72076 Tübingen, Germany

Department of Physics, University of Regensburg 8 , 93053 Regensburg, Germany

Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP) and Würzburg-Dresden Cluster of Excellence ct.qmat 9 , Technische Universität Dresden, 01062 Dresden, Germany

Department of Physics, Technical University of Munich 10 , 85748 Garching, Germany

Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling 11 ,’ Kekulestr. 5, 12489 Berlin, Germany

Carl von Ossietzky Universität Oldenburg, Institute of Physics 12 , Carl-von-Ossietzky-Straße 9, 26129 Oldenburg, Germany

Institute for Photovoltaics (ipv), University of Stuttgart 13 , Pfaffenwaldring 47, 70569 Stuttgart, Germany and , 52425 Jülich, Germany

Helmholtz Young Investigator Group, lEK5-Photovoltaik, Forschungszentrum Jülich 13 , Pfaffenwaldring 47, 70569 Stuttgart, Germany and , 52425 Jülich, Germany

Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden 14 , 01062 Dresden, Germany

Department of Physics and Materials Science, University of Luxembourg 15 , Luxembourg, Luxembourg

IEK5-Photovoltaik, Forschungszentrum Jülich 16 , 52425 Jülich, Germany and , Carl-Benz-Str. 199, 47057 Duisburg, Germany

Faculty of Engineering and CENIDE, University of Duisburg-Essen 16 , 52425 Jülich, Germany and , Carl-Benz-Str. 199, 47057 Duisburg, Germany

Institute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany

Freiburg Materials Research Center (FMF), University of Freiburg 18 , Stefan-Meier-Str. 21, 79104 Freiburg, Germany

Department of Organic and Perovskite Photovoltaics, Fraunhofer Institute for Solar Energy Systems (ISE) 19 , Heidenhofstraße 2, 79110 Freiburg, Germany

Applied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth 20 , 95440 Bayreuth, Germany

Bavarian Polymer Institute, University of Bayreuth 21 , 95440 Bayreuth, Germany

Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt 22 , Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany

Lehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU) 23 , Staudtstr. 7, 91058 Erlangen, Germany

Funding

Deutsche Forschungsgemeinschaft · Advanced Studies of the TU Munich · Bayerisches Staatsministerium: Wissenschaft und Kunst

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