journal article·2023-03-01Open access

Interlayer hybridization in a van der Waals quantum spin-Hall insulator/superconductor heterostructure

Fabio Bussolotti, Hiroyo Kawai, Ivan Verzhbitskiy, Wei Tao, Duc-Quan Ho, Anirban Das, Junxiang Jia, Shantanu Mukherjee, Bent Weber, Kuan Eng Johnson Goh

AIP Advances· Volume 13· Issue 3

Abstract

In this work, we present an angle-resolved photoemission spectroscopy study of a 1T′-WTe2 monolayer epitaxially grown on NbSe2 substrates, a prototypical quantum spin Hall insulator (QSHI)/superconductor heterojunction. Angle-resolved photoemission spectroscopy data indicate the formation of electronic states in the bulk bandgap of WTe2, which are absent in the nearly free-standing WTe2 grown on the highly oriented pyrolytic graphite substrate, where an energy gap of ∼100 meV is reported. The results are explained in terms of hybridization effects promoted by the QSHI–superconductor interaction at WTe2/NbSe2 interfaces, in line with recent scanning probe microscopy investigation and theoretical band structure calculations. Our findings highlight the important role of interlayer interaction on the electronic properties and ultimately on the engineering of topological properties of the QSHI/superconducting heterostructure.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Topological Materials and Phenomena · Graphene research and applications · 2D Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Institute of Materials Research and Engineering, Agency for Science Technology and Research (A∗STAR) 1 , 2 Fusionopolis Way, #08-03 Innovis, Singapore 138634, Republic of Singapore

Institute of High Performance Computing, Agency for Science, Technology and Research 2 , 1 Fusionopolis Way, #16-16 Connexis, Singapore 138632, Republic of Singapore

Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University 3 , 50 Nanyang Avenue, 639798, Singapore

Department of Physics, Indian Institute of Technology Madras 4 , Chennai 600036, India

Department of Physics, National University of Singapore 5 , 2 Science Drive 3, Singapore 117551, Singapore

Funding

National Research Foundation Singapore · Agency for Science, Technology and Research

References (22)

Show source-provided references
1. Atomically thin quantum spin Hall insulators10.1002/adma.202008029 ↗
2. Quantum spin Hall effect and enhanced magnetic response by spin-orbit coupling10.1103/physrevlett.97.236805 ↗
3. Topological superconductors: A review10.1088/1361-6633/aa6ac7 ↗
4. Superconducting proximity effect and Majorana fermions at the surface of a topological insulator10.1103/physrevlett.100.096407 ↗
5. New directions in the pursuit of Majorana fermions in solid state systems10.1088/0034-4885/75/7/076501 ↗
6. Engineered platforms for topological superconductivity and Majorana zero modes10.1038/s41578-021-00336-6 ↗
7. Proximity-induced superconducting gap in the quantum spin Hall edge state of monolayer WTe210.1038/s41567-020-0816-x ↗
8. Multiband superconductivity in strongly hybridized 1T′-WTe2/NbSe2 heterostructures10.1103/physrevb.105.094512 ↗
9. Van der Waals heterostructures10.1038/nature12385 ↗
10. Electronic structural Moiré pattern effects on MoS2/MoSe2 2D heterostructures10.1021/nl4030648 ↗
11. Photonic crystals for nano-light in Moiré graphene superlattices10.1126/science.aau5144 ↗
12. 2D materials and van Der Waals heterostructures10.1126/science.aac9439 ↗
13. Angle-resolved photoemission studies of the cuprate superconductors10.1103/revmodphys.75.473 ↗
14. Quantum spin Hall State in monolayer 1T′-WTe210.1038/nphys4174 ↗
15. Colloquium: Graphene spectroscopy10.1103/revmodphys.86.959 ↗
16. Protected hole valley states in single-layer MoS210.1103/physrevb.99.045134 ↗
17. Electronic properties of atomically thin MoS2 layers grown by physical vapour deposition: Band structure and energy level alignment at layer/substrate interfaces10.1039/c8ra00635k ↗
18. Quantitative electron spectroscopy of surfaces: A standard data base for electron inelastic mean free paths in solids10.1002/sia.740010103 ↗
19. Evidence for magnetic weyl fermions in a correlated metal10.1038/nmat4987 ↗
20. Nanoscale studies of electric field effects on monolayer 1T′-WTe210.1038/s41535-022-00433-x ↗
21. Impact of S-vacancies on the charge injection barrier at the electrical contact with the MoS2 monolayer10.1021/acsnano.0c07982 ↗
22. Coulomb disorder effects on angle-resolved photoemission and nuclear quadrupole resonance spectra in cuprates10.1103/physrevb.80.094519 ↗