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journal article·2019-10-01Open access

Measurement of the third order nonlinear susceptibility of paratellurite single crystal using multiplex CARS

Zakaniaina Rajaofara, Philippe Leproux, Erwan Capitaine, Hideaki Kano, Tomokatsu Hayakawa, Philippe Thomas, Jean-René Duclère, Vincent Couderc

AIP Advances· Volume 9· Issue 10
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Source abstract

Abstract

We report the extraction of the real part of the third order nonlinear susceptibility for a c-cut paratellurite (TeO2 − α) single crystal using the nonresonant contribution of the multiplex coherent anti-Stokes Raman scattering (M-CARS) signal. Using fused silica and SF57 as nonlinear reference materials, we derive the absolute value of the real part of the electronic third order susceptibility and we evidence the in-plane modulation of the nonlinear refractive index. These results are in total agreement with those recently obtained by the z-scan method.
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Research context

OpenAlex topics: Spectroscopy Techniques in Biomedical and Chemical Research · Photorefractive and Nonlinear Optics · Advanced Fiber Laser Technologies

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Affiliations

Institut de Recherche sur les Céramiques, UMR 7315 CNRS-Université de Limoges, Centre Européen de la Céramique 1 , 12, rue Atlantis, 87068 Limoges Cedex, France

Institut XLIM, UMR 7252 CNRS – Université de Limoges 2 , 123, Avenue Albert Thomas, 87060 Limoges Cedex, France

Department of Applied Physics, Graduate School of Pure and Applied Sciences, University of Tsukuba 3 , 1-1-1 Tennodai, Tsukuba, Ibaraki, 305-8573, Japan

Field of Advanced Ceramics, Department of Life Science and Applied Chemistry, Nagoya Institute of Technology 4 , Gokiso, Showa, Nagoya 466-8555, Japan

Funding

French ANR/TRAFIC Project · French Defense Agency/French ANR · Région Nouvelle-Aquitaine NEMATUUM

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