journal article·2024-02-01Open access

Enhanced orbital magnetic moment of Co film grown on Fe3O4(001)

Zhe Zhang, Xianyang Lu, Zhihao Li, Zhuoyi Li, Yu Yan, Yuzhe Chen, Jun Du, Fangyuan Zhu, Jiefeng Cao, Yong Wang, Yao Li, Liang He, Jing Wu, Rong Zhang, Yongbing Xu

AIP Advances· Volume 14· Issue 2

Abstract

We investigate the magnetic and electronic properties of Co films on Fe3O4(001) achieved through epitaxial growth using magnetron sputtering. X-ray magnetic circularly dichroism measurements characterize the atomic magnetism. Compared to Co films on the MgO substrate, Co on Fe3O4 exhibits a 96% enhancement in orbital magnetic moment (from 0.25 to 0.49 µB/atom) and an increase in spin magnetic moment (from 1.37 to 1.53 µB/atom), resulting in an increased mratio(ml/ms) from 0.18 to 0.32. This enhancement of the orbital moment emerges as a consequence of the interface interaction between Co and Fe3O4. Density functional theory calculations attribute this heightened orbital magnetic moment to the robust electronic exchange interactions. Our findings not only offer insights into the modulation of magnetic and electronic characteristics in Co-based magnetic heterostructures but also provide valuable implications for the potential application of magnetic oxide/ferromagnetic heterostructures in future spintronic devices.
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Research context

OpenAlex topics: Magnetic properties of thin films · Magnetic Properties and Synthesis of Ferrites · Advanced Condensed Matter Physics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials, School of Electronic Science and Engineering, Nanjing University 1 , Nanjing 210093, China

School of Integrated Circuits, Nanjing University 2 , Suzhou 215163, China

Department of Physics, Nanjing University 3 , Nanjing 210093, China

Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences 4 , Shanghai 201204, China

York-Nanjing International Joint Center in Spintronics, Department of Electronics and Physics, University of York 5 , York YO10 5DD, United Kingdom

Funding

National Key Research and Development Program of China · National Natural Science Foundation of China · Natural Science Foundation of Jiangsu Province

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