Robust method for broadband efficiency enhancement of electron photocathodes using optical interferences
Source abstract
Abstract
We demonstrate the key features of an interference cathode using both simulations and experiments. We deposit Cs3Sb photocathodes on Ag to produce an interference enhanced photocathode with 2–5× quantum efficiency (QE) enhancement using a robust procedure that requires only a smooth metal substrate and QE monitoring during growth. We grow both an interference cathode (Ag substrate) and a typical photocathode (Si reference substrate) simultaneously to confirm that the effects are due to optical interactions with the substrate rather than photocathode composition or surface electron affinity differences. Growing the cathodes until the QE converges shows both the characteristic interference peaks during growth and the identical limiting case where the cathode is “infinitely thick,” in agreement with simulations. We also grow a cathode until the QE on Ag peaks and then stop the growth, demonstrating broadband QE enhancement.
Source: crossref · Quality: baseline
Research context
OpenAlex topics: Photocathodes and Microchannel Plates · Electron and X-Ray Spectroscopy Techniques · Advanced Chemical Physics Studies
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
Los Alamos National Laboratory 1 , Mailstop H851, Los Alamos, New Mexico 87545, USA
Brookhaven National Laboratory 2 , Building 535-B, Upton, New York 11973, USA
Helmholtz-Zentrum Berlin 3 , Albert-Einstein Strasse 15, Berlin 12489, Germany
Funding
Los Alamos National Laboratory
References (34)
Show source-provided references
1. Grand challenges in basic energy sciences10.1063/1.2963009 ↗
2. Photocathodes—Past performance and future potential10.1080/00107510302717 ↗
3. Simulation of large photomultipliers for experiments in astroparticle physics10.1016/j.nima.2009.11.023 ↗
4. Photoemission sources and beam blankers for ultrafast electron microscopy10.1063/1.5117058 ↗
5. Perspectives on designer photocathodes for x-ray free-electron lasers: Influencing emission properties with heterostructures and nanoengineered electronic states10.1103/physrevapplied.10.047002 ↗
6. Photoemission experiments of a large area scandate dispenser cathode10.1016/j.nima.2010.05.026 ↗
7. Electron induction linacs10.1007/978-3-642-13917-8_7 ↗
8. Seitz · 201110.1007/978-3-642-18443-7 ↗
9. Single-photon imaging detector with O(10) ps timing and sub-10 μm position resolutions10.1088/1748-0221/13/12/c12005 ↗
10. Advances in bright electron sources10.1016/j.nima.2018.03.019 ↗
11. Modern theory and applications of photocathodes10.1117/12.158575 ↗
12. Sources of emittance in RF photocathode injectors: Intrinsic emittance, space charge forces due to non-uniformities, RF and solenoid effects
13. Reduction of intrinsic electron emittance from photocathodes using ordered crystalline surfaces10.1103/physrevlett.118.164802 ↗
14. Synthesis and x-ray characterization of sputtered bi-alkali antimonide photocathodes10.1063/1.5010950 ↗
15. Enhanced quantum efficiency of photoelectron emission, through surface textured metal electrodes10.1116/1.4936082 ↗
16. Record-level quantum efficiency from a high polarization strained GaAs/GaAsP superlattice photocathode with distributed Bragg reflector10.1063/1.4972180 ↗
17. Surface-plasmon resonance-enhanced multiphoton emission of high-brightness electron beams from a nanostructured copper cathode10.1103/PhysRevLett.110.074801 ↗
18. Effects of surface nonuniformities on the mean transverse energy from photocathodes10.1103/physrevapplied.4.024015 ↗
19. Ultra low emittance electron beams from multi-alkali antimonide photocathode operated with infrared light10.1063/1.4945091 ↗
20. Enhanced photocathode performance through optimization of film thickness and substrate10.1116/1.4976527 ↗
21. 2015
22. Degree of roughness of rough layers: extensions of the Rayleigh roughness criterion and some applications10.2528/PIERB09110907 ↗
23. Near atomically smooth alkali antimonide photocathode thin films10.1063/1.4974363 ↗
24. Bi-alkali antimonide photocathodes for high brightness accelerators10.1063/1.4821625 ↗
25. Thickness dependence of the quantum yield of cesium-antimony films10.1002/pssb.19680270115 ↗
26. Analysis of a multiple reflective translucent photocathode10.1364/ao.6.000443 ↗
27. Optical means for enhancing the sensitivity of a tri-alkali photocathode10.1364/ao.6.001171 ↗
28. Theory of photoemission from cesium antimonide using an alpha-semiconductor model10.1063/1.2967826 ↗
29. Optical constants of the noble metals10.1103/physrevb.6.4370 ↗
30. Temperature dependence of the dielectric function of silicon using in situ spectroscopic ellipsometry10.1016/0040-6090(93)90082-z ↗
31. See https://www.mtixtl.com/Mc-Ag-a-050505S1.aspx for Ag (Silver) Single Crystal Substrate: 〈100〉, 5 × 5 × 0.5 mm, 1 side polished—McAga050505S1; accessed 23 May 2021.
32. Codeposition of ultrasmooth and high quantum efficiency cesium telluride photocathodes10.1103/physrevaccelbeams.22.073401 ↗
33. In-situ synchrotron x-ray characterization of K2CsSb photocathode grown by ternary co-evaporation10.1063/1.4975113 ↗
34. Commentary: The materials project: A materials genome approach to accelerating materials innovation10.1063/1.4812323 ↗