journal article·2024-12-01Open access

Synergistic effect mechanism of the core state, surface state, and solvent relaxation of N-doped red carbon dots

Taiqun Yang, Huangmei Zhou, Yu Zhao, Wenhui Yang, Lei Li, Chaoqun Ma, Menghui Jia, Guoqing Chen, Sanjun Zhang

AIP Advances· Volume 14· Issue 12

Abstract

Nitrogen-doping carbon dots have attracted broad interest in recent years due to their excellent spectral properties and promising applications. However, the luminescence mechanism of these carbon dots still lacks support from time-resolved spectroscopy. In this work, carbon dots were synthesized using p-phenylenediamine as a precursor (p-CDs), and their excited state dynamics were studied using transient absorption and time-resolved fluorescence spectroscopy. Experimental results reveal the origins of dual fluorescence and the synergistic effect mechanism involving the core state, the surface state, and solvent relaxation. Fluorescence lifetime imaging of p-CDs was performed in cells, highlighting their great potential for applications in biological fields.
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Research context

OpenAlex topics: Carbon and Quantum Dots Applications · Nanocluster Synthesis and Applications · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

School of Science, Jiangnan University 1 , Wuxi 214122,

Jiangsu Provincial Research Center of Light Industrial Optoelectronic Engineering and Technology 2 , Wuxi 214122,

State Key Laboratory of Precision Spectroscopy, East China Normal University 3 , Shanghai 200241,

Materials Characterization Center, Multifunctional Platform for Innovation, East China Normal University 4 , Shanghai 200241,

Collaborative Innovation Center of Extreme Optics, Shanxi University 5 , Taiyuan, Shanxi 030006,

Funding

National Natural Science Foundation of China

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