journal article·2025-06-01Open access

Room-temperature spin-glass behaviors and memory effects in Al-substituted Y3Fe5O12 epitaxial film grown by pulsed laser deposition

Takahiro Yoshino, Siyi Tang, Md Shamim Sarker, EMK Ikball Ahamed, Zhiqiang Liao, Hiroyasu Yamahara, Hitoshi Tabata, Munetoshi Seki

AIP Advances· Volume 15· Issue 6

Abstract

This study explores the magnetic properties of a thin film of Al-substituted Y3Fe5O12 grown on Y3Al5O12 (111) substrates using pulsed laser deposition. Spin-glass behavior was observed near room temperature in the film, with a spin-freezing temperature of 345 K achieved. This temperature is significantly higher than those previously reported for spin-glass systems based on Fe oxides. The film exhibited characteristic memory and rejuvenation effects below the spin-freezing temperature, which are explained by magnetic relaxation via metastable states within a multi-valley energy landscape featuring shallow activation energies. Additionally, photomagnetic memory effects were demonstrated using the magneto-optic effect of the film at room temperature. Our results highlight the potential application of the Al-substituted Y3Fe5O12 film in neuromorphic devices with low energy consumption.
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Research context

OpenAlex topics: Theoretical and Computational Physics · Transition Metal Oxide Nanomaterials · Metallic Glasses and Amorphous Alloys

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Electrical Engineering and Information Systems, Graduate School of Engineering, The University of Tokyo 1 , 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656,

Department of Bioengineering, Graduate School of Engineering, The University of Tokyo 2 , 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656,

Center for Spintronics Research Network (CSRN), Graduate School of Engineering, The University of Tokyo 3 , 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656,

Funding

Core Research for Evolutional Science and Technology · Japan Society for the Promotion of Science · Japan Agency for Medical Research and Development

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