Strategy of Triple‐Gradient in Binary Pixels for Flexible Pressure Sensing with High Sensitivity and Wide‐Range Linearity

ABSTRACT Flexible pressure sensors have recently aroused increasing interests for fields of electronic skin, intelligent robotics, and human‐machine interactions (HMI). Preserving high sensitivity of flexible pressure sensors across a broad range is essential prerequisite to ensure signal‐to‐noise reliability for multiple applications. However, this remains challenging due to the inherent sensing saturation when flexible matrix is exposed to varying pressure. Herein, a flexible pressure sensor based on design of binary micro‐dome pixels is proposed. Triple‐gradient of conductivity, modulus, and dimension is precisely designed in binary pixels, ensuring mechanical and electrical compensation during the entire deformation process. With well‐developed CNT/PDMS matrix, significant sensing enhancement is realized, showcasing a linear sensitivity of 974.1 kPa ⁻¹ across range up to 1.8 MPa (R ² > 0.99). Thanks to the preserved sensitivity, the wearable device can recognize body information such as pulse, joint motion, and even foot pressure. The broad linearity also allows HMI establishment that applies force level as one basic clue to reflect human intension, e.g. dual‐factor authentication system. Along with superiorities of low detection limit, fast response, and mechanical robustness, the principle of triple‐gradient in binary pixels can be of significance for development of high‐performance flexible sensors in the future is expected.