journal article·2019-11Open access

CO2 Photoreduction: Heterostructure Engineering of a Reverse Water Gas Shift Photocatalyst (Adv. Sci. 22/2019)

Hong Wang, Jia Jia, Lu Wang, Keith Butler, Rui Song, Gilberto Casillas, Le He, Nazir P. Kherani, Doug D. Perovic, Liqiang Jing, Aron Walsh, Roland Dittmeyer, Geoffrey A. Ozin

Advanced Science· Volume 6· Issue 22

Abstract

In article number 1902170, Hong Wang, Geoffrey A. Ozin, and co-workers present a hetero-nanostructure, oxygen vacancy, electronic band alignment and carrier lifetime engineering strategy of In2O3−x(OH)y@Nb2O5, enabling the solar-powered, reverse water gas shift reaction to operate at a 44-fold higher conversion rate than pristine In2O3−x(OH)y, with high selectivity and long-term operational stability, an advance that augers well for the metal oxide hetero-nanostructure engineering approach to the industrialization of gas-phase CO2 photocatalysis. Image credit: Chenxi Qian.
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Research context

OpenAlex topics: Advanced Photocatalysis Techniques

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Affiliations

Key Laboratory of Functional Polymer Materials of the Ministry of Education Institute of Polymer Chemistry College of Chemistry Nankai University Tianjin 300071 P. R. China

Materials Chemistry and Nanochemistry Research Group Solar Fuels Cluster Departments of Chemistry University of Toronto 80 St. George Street Toronto ON M5S3H6 Canada

Department of Materials Science and Engineering University of Toronto 184 College Street Toronto ON M5S3E4 Canada

Institute of Functional Nano & Soft Materials (FUNSOM) Jiangsu Key Laboratory for Carbon‐Based Functional Materials & Devices Soochow University 199 Ren'ai Road Suzhou Jiangsu P. R. China

SciML, Scientific Computing Department, Rutherford Appleton Laboratory Didcot OX110QX UK

UOW Electron Microscopy Centre, University of Wollongong Wollongong New South Wales 2500 Australia

Key Laboratory of Functional Inorganic Material Chemistry Ministry of Education School of Chemistry and Materials Science International Joint Research Center for Catalytic Technology Heilongjiang University Harbin 150080 P. R. China

Department of Materials, Imperial College London Exhibition Road London SW7 2AZ UK

Department of Materials Science and Engineering, Yonsei University Seoul 03722 Korea

Institute for Micro Process Engineering, Karlsruhe Institute of Technology Hermann‐von‐Helmholtz‐Platz 1 76344 Eggenstein‐Leopoldshafen Germany

References

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