journal article·2026-05Open access

Superradiance and Broadband Emission Driving Fast Electron Dephasing in Open Quantum Systems

Gimin Bae, Youngjae Kim, Jae Dong Lee

Advanced Science· Volume 13· Issue 27

Abstract

ABSTRACT The physical origin of the ultrashort dephasing time T 2 (≈ O(1) fs), persistently addressed in the solid‐state high‐harmonic generation (HHG), remains an unresolved and challenging issue because the electron scattering at such a short timescale within solids is hardly identified. Here we investigate HHG of the 1D Hubbard model in the dissipative quantum environment within a frame of the Lindblad equation. In the study, in the limit of a small interatomic distance, we make the first verification of the solid‐state Dicke superradiance, the coherent stimulated emission triggered by the spontaneous emission, as well as the broadband emission mimicking the blackbody radiation due to the electron scattering in each harmonic multiple. Further, we find a strong destructive interference between the Dicke superradiance and the broadband emission, which makes a scale down of the effective electron scattering time and leads to just few‐femtosecond dephasing time T 2 . This finding explains a long‐standing problem of the ultrafast femtosecond electron dephasing in HHG. The present study could also serve as a pertinent platform for understanding the nonequilibrium dissipative dynamics of correlated electron systems.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Laser-Matter Interactions and Applications · Spectroscopy and Quantum Chemical Studies · Nonlinear Photonic Systems

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Physics and Chemistry DGIST Daegu Republic of Korea

School of Physics KIAS Seoul Republic of Korea

Funding

National Research Foundation of Korea · Ministry of Science and ICT, South Korea

References (44)

Show source-provided references
1. 10.1038/s41567‐018‐0315‐510.1038/s41567‐018‐0315‐5 ↗
2. 10.1103/PhysRevLett.80.374310.1103/PhysRevLett.80.3743 ↗
3. 10.1103/PhysRevA.94.03341010.1103/PhysRevA.94.033410 ↗
4. 10.1103/PhysRevLett.115.19360310.1103/PhysRevLett.115.193603 ↗
5. 10.1364/OPTICA.4.00051610.1364/OPTICA.4.000516 ↗
6. 10.1103/PhysRevLett.118.08740310.1103/PhysRevLett.118.087403 ↗
7. 10.1038/s41566‐022‐01010‐110.1038/s41566‐022‐01010‐1 ↗
8. 10.1103/PhysRevB.103.L16140610.1103/PhysRevB.103.L161406 ↗
9. 10.1038/nphys394610.1038/nphys3946 ↗
10. 10.1038/s41467‐018‐03397‐410.1038/s41467‐018‐03397‐4 ↗
11. 10.1088/1361‐6455/abb12710.1088/1361‐6455/abb127 ↗
12. 10.1007/978-1-4612-1470-010.1007/978-1-4612-1470-0 ↗
13. 10.1038/s41467‐022‐34337‐y10.1038/s41467‐022‐34337‐y ↗
14. 10.1364/OPTICA.44410510.1364/OPTICA.444105 ↗
15. 10.1021/acs.nanolett.3c0427810.1021/acs.nanolett.3c04278 ↗
16. 10.1103/PhysRevLett.125.08390110.1103/PhysRevLett.125.083901 ↗
17. 10.1103/PhysRevLett.113.07390110.1103/PhysRevLett.113.073901 ↗
18. 10.1103/PhysRevA.97.01140110.1103/PhysRevA.97.011401 ↗
19. 10.1103/PhysRevResearch.6.04300510.1103/PhysRevResearch.6.043005 ↗
20. 10.1103/PhysRevLett.121.09740210.1103/PhysRevLett.121.097402 ↗
21. 10.1073/pnas.220421911910.1073/pnas.2204219119 ↗
22. 10.1038/s41566‐019‐0516‐110.1038/s41566‐019‐0516‐1 ↗
23. 10.1038/s41566‐018‐0129‐010.1038/s41566‐018‐0129‐0 ↗
24. 10.1103/PhysRevLett.132.18690110.1103/PhysRevLett.132.186901 ↗
25. 10.1103/PhysRevA.90.02361810.1103/PhysRevA.90.023618 ↗
26. 10.1016/0370‐1573(82)90102‐810.1016/0370‐1573(82)90102‐8 ↗
27. 10.1103/PhysRevA.2.88910.1103/PhysRevA.2.889 ↗
28. 10.1103/PRXQuantum.5.01034410.1103/PRXQuantum.5.010344 ↗
29. 10.1038/s41467‐022‐29805‐410.1038/s41467‐022‐29805‐4 ↗
30. 10.1103/PhysRevB.103.L04140810.1103/PhysRevB.103.L041408 ↗
31. 10.34133/2021/982071610.34133/2021/9820716 ↗
32. 10.1103/PhysRevB.107.19510310.1103/PhysRevB.107.195103 ↗
33. 10.1103/PhysRevLett.116.01660110.1103/PhysRevLett.116.016601 ↗
34. 10.1103/PhysRevB.86.07514810.1103/PhysRevB.86.075148 ↗
35. 10.1103/PhysRevB.106.23514210.1103/PhysRevB.106.235142 ↗
36. 10.1103/PhysRevLett.127.06040310.1103/PhysRevLett.127.060403 ↗
37. 10.1103/PhysRevLett.131.06360110.1103/PhysRevLett.131.063601 ↗
38. 10.1103/PhysRevA.94.02381910.1103/PhysRevA.94.023819 ↗
39. 10.1126/science.117669510.1126/science.1176695 ↗
40. 10.1021/nl401474810.1021/nl4014748 ↗
41. 10.1038/s41586‐024‐07156‐y10.1038/s41586‐024‐07156‐y ↗
42. 10.1103/PhysRevB.92.20510810.1103/PhysRevB.92.205108 ↗
43. 10.1103/PhysRevB.109.12510810.1103/PhysRevB.109.125108 ↗
44. 10.1103/PhysRevB.106.20542210.1103/PhysRevB.106.205422 ↗