Interplay between Spin‐Orbit Torques and Dzyaloshinskii‐Moriya Interactions in Ferrimagnetic Amorphous Alloys

Abstract Ferrimagnetic thin films are attractive for low‐power spintronic applications because of their low magnetization, small angular momentum, and fast spin dynamics. Spin orbit torques (SOT) can be applied with proximal heavy metals that also generate interfacial Dzyaloshinskii–Moriya interactions (DMI), which can stabilize ultrasmall skyrmions and enable fast domain wall motion. Here, the properties of a ferrimagnetic CoGd alloy between two heavy metals to increase the SOT efficiency, while maintaining a significant DMI is studied. SOT switching for various capping layers and alloy compositions shows that Pt/CoGd/(W or Ta) films enable more energy‐efficient SOT magnetization switching than Pt/CoGd/Ir. Spin‐torque ferromagnetic resonance confirms that Pt/CoGd/W has the highest spin‐Hall angle of 16.5%, hence SOT efficiency, larger than Pt/CoGd/(Ta or Ir). Density functional theory calculations indicate that CoGd films capped by W or Ta have the largest DMI energy, 0.38 and 0.32 mJ m⁻², respectively. These results show that Pt/CoGd/W is a very promising ferrimagnetic structure to achieve small skyrmions and to move them efficiently with current.