journal article·2025-01Open access

Organophotocatalyst Enabled Deoxycyclopropanation of Alcohols

Yongsheng Zhang, Jincheng Wang, Xiaoyan He, Shilin Peng, Lei Yuan, Gang Huang, Yongjin Guo, Xiuhong Lu

Advanced Science· Volume 12· Issue 1

Abstract

Abstract Cyclopropane fragments, which widely exist in marketed drugs and natural products, can confer special pharmacological properties to small‐molecule drugs. Therefore, developing methods to construct cyclopropanes is of great significance. Nevertheless, the introduction of cyclopropane primarily relies on already‐formed cyclopropyl groups, which significantly restricts the diversity of cyclopropane skeletons. Late‐stage direct cyclopropanation is still a challenging task. Herein, a photo‐induced intermolecular deoxycyclopropanation reaction that employs alcohols as substrates, and 1 mol.% of 2,3,5,6‐tetrakis(carbazol‐9‐yl)‐1,4‐dicyanobenzene (4CzTPN) as organophotocatalyst is reported. This method proceeds with high transformation efficiency (up to 98% yield) and exhibits broad functional group tolerance, such as primary, secondary, and tertiary alcohols as well as various activated β‐halogenated alkenes. This process is mild, easy to operate, and has low equipment requirements. The power of this technology is demonstrated by the late‐stage functionalization of five marketed drugs and five natural products.
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Research context

OpenAlex topics: Cyclopropane Reaction Mechanisms · Catalytic C–H Functionalization Methods · Radical Photochemical Reactions

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Shanghai Key Laboratory of Molecular Imaging Jiading District Central Hospital Affiliated Shanghai University of Medicine and Health Sciences Shanghai 201318 P. R. China

Key Laboratory of Structure‐Based Drug Design & Discovery of Ministry of Education Shenyang Pharmaceutical University Shenyang 110016 P. R. China

School of Pharmacy Shanghai University of Medicine and Health Sciences Shanghai 201318 P. R. China

Funding

National Natural Science Foundation of China · Shanghai Key Laboratory of Molecular Imaging · National Key Research and Development Program of China

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