journal article·2022-10

Energy‐Controllable Exciton‐Polariton Bose–Einstein Condensation in Perovskite Microstrip Cavities

Ang Ren, Ji Tang, Zhengjun Jiang, Yongli Yan, Jiannian Yao, Yong Sheng Zhao

Advanced Optical Materials· Volume 10· Issue 19
Publisher page

Abstract

Abstract Manipulating exciton‐polaritons (EPs) to condense into different energy states is critically important for the development of polariton‐related fundamental mechanisms and functional devices. Although various schemes are proposed for this purpose, exploiting tunable traps originating from the structure itself suffers from concomitant nonradiative recombination and dephasing effects, which limits the investigation of polariton physics and hinders their application in polaritonic devices. Here, a strategy to achieve energy‐controllable EP Bose–Einstein condensation in rationally designed low‐dimensional perovskite microcavities based on the lateral confinement and ballistic propagation of polariton condensates is demonstrated. Perovskite single‐crystal microstrips with finite lateral size provide multiple discrete polariton states. The distribution of polariton condensates among different energy states is effectively modulated by means of EP propagation in perovskite microstrips. With this new concept, stable polariton lasing with excellent wavelength‐switchability is realized. These results offer useful insight into using 1D polariton systems to construct all‐optical polaritonic circuit applications at room temperature.
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Research context

OpenAlex topics: Strong Light-Matter Interactions · Thermal Radiation and Cooling Technologies · Perovskite Materials and Applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Key Laboratory of Photochemistry Institute of Chemistry Chinese Academy of Sciences Beijing 100190 P. R. China

University of Chinese Academy of Sciences Beijing 100049 P. R. China

Funding

National Natural Science Foundation of China · Natural Science Foundation of Beijing Municipality

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