journal article·2018-01Open access

Continuous‐Wave Lasing in Cesium Lead Bromide Perovskite Nanowires

Tyler J. S. Evans, Andrew Schlaus, Yongping Fu, Xinjue Zhong, Timothy L. Atallah, Michael S. Spencer, Louis E. Brus, Song Jin, X.‐Y. Zhu

Advanced Optical Materials· Volume 6· Issue 2

Abstract

Abstract Lead halide perovskite nanowires (NWs) have been demonstrated in pulsed lasing with high quantum yields, low thresholds, and broad tunability. However, continuous‐wave (CW) lasing, necessary for many optoelectronic applications, has not been achieved to date. This is thought to be due to many‐body screening, which reduces the excitonic resonance enhancement of the oscillator strength at high excitation densities necessary for population inversion. Here CW lasing in CsPbBr3 perovskite NWs is reported. Analysis of the cavity modes and their temperature dependence reveals that both CW and pulsed lasing originate from polariton modes near the bottleneck region on the lower polariton branch, with a vacuum Rabi splitting of 0.20 ± 0.03 eV. These findings suggest that lead halide perovskite NWs may serve as low‐power CW coherent light sources and as model systems for polaritonics in the strong‐coupling regime.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Strong Light-Matter Interactions · Thermal Radiation and Cooling Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Chemistry Columbia University New York NY 10027 USA

Department of Chemistry University of Wisconsin‐Madison Madison WI 53706 USA

Funding

U.S. Department of Energy

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