Shortwave Infrared Light Detection and Ranging Using Silver Telluride Quantum Dots
Source abstract
Abstract
Abstract Shortwave infrared (SWIR) light, characterized as the “eye‐safe” window, is considered extremely promising in various technological fields and particularly valuable for imaging and light detection and ranging (LiDAR) applications. Silver telluride (Ag 2 Te) colloidal quantum dots (CQDs), featuring RoHS‐compliance, solution‐processability, and CMOS compatibility, emerge as a potential contender for SWIR optoelectronics. Yet, further improvements in dark current, response speed, and linear dynamic range (LDR) are essential for meeting the rigorous demands of sensing and LiDAR applications. Here, it is shown that post‐synthesis surface engineering and doping control significantly improve the dark current, response speed, and LDR of Ag₂Te CQD photodiodes, achieving a low dark current of 450 nA cm − 2 at −0.5 V, an LDR exceeding 150 dB, and a rapid response speed of ≈25 ns. A proof‐of‐concept LiDAR demonstration in the SWIR using a practical nanosecond diode laser achieves decimetre‐level resolution at a distance exceeding 10 m. This work represents a key step in advancing SWIR CQDs toward consumer electronics and automotive markets.
Source: crossref · Quality: baseline
Research context
OpenAlex topics: Quantum Dots Synthesis And Properties · Chalcogenide Semiconductor Thin Films · Perovskite Materials and Applications
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
The Barcelona Institute of Science and Technology ICFO‐Insitut de Ciencies Fotoniques Castelldefels Barcelona 08860 Spain
ICREA‐Institució Catalana de Recerca i Estudiats Avançats Lluis Companys 23 Barcelona 08010 Spain
Funding
European Research Council · European Commission · Agencia Estatal de Investigación
References (56)
Show source-provided references
1. 10.1016/0004-6981(69)90045-610.1016/0004-6981(69)90045-6 ↗
2. 10.1021/acsnano.4c1178710.1021/acsnano.4c11787 ↗
3. 10.1016/S0042-6989(96)00120-410.1016/S0042-6989(96)00120-4 ↗
4. 10.1002/adma.20240200210.1002/adma.202402002 ↗
5. 10.1021/acsnano.4c0655910.1021/acsnano.4c06559 ↗
6. 10.1038/nmat129910.1038/nmat1299 ↗
7. 10.1038/s41467-019-13158-610.1038/s41467-019-13158-6 ↗
8. 10.1038/nature0485510.1038/nature04855 ↗
9. 10.1021/acs.nanolett.2c0095010.1021/acs.nanolett.2c00950 ↗
10. 10.1002/adfm.20240530710.1002/adfm.202405307 ↗
11. 10.1038/s41566-019-0362-110.1038/s41566-019-0362-1 ↗
12. 10.1021/jacs.4c0620210.1021/jacs.4c06202 ↗
13. 10.1002/adma.20230184210.1002/adma.202301842 ↗
14. 10.1021/jacs.4c1075510.1021/jacs.4c10755 ↗
15. 10.1002/adma.20220303910.1002/adma.202203039 ↗
16. 10.1002/adma.20230614710.1002/adma.202306147 ↗
17. 10.1021/acsnano.3c1200710.1021/acsnano.3c12007 ↗
18. 10.1002/advs.20230643910.1002/advs.202306439 ↗
19. 10.1002/advs.20240745310.1002/advs.202407453 ↗
20. 10.1021/acsmaterialslett.4c0158510.1021/acsmaterialslett.4c01585 ↗
21. 10.1038/s41566-023-01345-310.1038/s41566-023-01345-3 ↗
22. 10.1021/acs.nanolett.3c0277010.1021/acs.nanolett.3c02770 ↗
23. 10.1021/acs.nanolett.4c0265910.1021/acs.nanolett.4c02659 ↗
24. 10.1038/s41928-022-00799-710.1038/s41928-022-00799-7 ↗
25. 10.1021/acsnano.5b0629510.1021/acsnano.5b06295 ↗
26. 10.1021/acsnano.4c0496810.1021/acsnano.4c04968 ↗
27. 10.1021/acs.accounts.3c0017410.1021/acs.accounts.3c00174 ↗
28. 10.1021/jacs.7b0015810.1021/jacs.7b00158 ↗
29. 10.1039/C9TA02393C10.1039/C9TA02393C ↗
30. 10.1002/smll.20230653510.1002/smll.202306535 ↗
31. 10.1002/advs.20150008810.1002/advs.201500088 ↗
32. 10.1021/accountsmr.0c0011110.1021/accountsmr.0c00111 ↗
33. Gregori L. · Small · 2024 · 20
34. 10.1016/j.joule.2020.07.00310.1016/j.joule.2020.07.003 ↗
35. 10.1126/science.aac552310.1126/science.aac5523 ↗
36. 10.1021/acsanm.3c0504310.1021/acsanm.3c05043 ↗
37. 10.1021/acsnano.3c0391110.1021/acsnano.3c03911 ↗
38. 10.1016/j.matt.2019.05.01510.1016/j.matt.2019.05.015 ↗
39. 10.1002/adma.20210753210.1002/adma.202107532 ↗
40. 10.1038/nnano.2015.24710.1038/nnano.2015.247 ↗
41. 10.1063/5.001980010.1063/5.0019800 ↗
42. 10.1021/nl301104z10.1021/nl301104z ↗
43. 10.1002/adfm.20221015810.1002/adfm.202210158 ↗
44. 10.1039/C6EE01577H10.1039/C6EE01577H ↗
45. 10.1063/1.282358210.1063/1.2823582 ↗
46. 10.1038/s41928-022-00779-x10.1038/s41928-022-00779-x ↗
47. 10.1021/acs.nanolett.4c0223510.1021/acs.nanolett.4c02235 ↗
48. 10.1002/adma.20242027310.1002/adma.202420273 ↗
49. 10.1021/acsenergylett.3c0251510.1021/acsenergylett.3c02515 ↗
50. 10.1002/ange.20231673310.1002/ange.202316733 ↗
51. 10.1016/j.matt.2020.12.01710.1016/j.matt.2020.12.017 ↗
52. 10.1038/s41586-024-07076-x10.1038/s41586-024-07076-x ↗
53. 10.1038/s41563-022-01204-610.1038/s41563-022-01204-6 ↗
54. 10.1021/acs.nanolett.1c0189210.1021/acs.nanolett.1c01892 ↗
55. 10.1002/adma.1997009030810.1002/adma.19970090308 ↗
56. 10.1038/s41586-024-07363-710.1038/s41586-024-07363-7 ↗