journal article·2023-11Open access

Continuous‐Wave Lasing in Perovskite LEDs with an Integrated Distributed Feedback Resonator

Kaichuan Wen, Yu Cao, Lianghui Gu, Saixue Wang, Dongmin Qian, Jingmin Wang, Zhiyuan Kuang, Mengyi Luo, Gang Wang, Shuzhen Guan, Mengmeng Li, Heng Yang, Guichuan Xing, Nana Wang, Lin Zhu, Qiming Peng, Wei Huang, Jianpu Wang

Advanced Materials· Volume 35· Issue 44

Abstract

Abstract Realization of electrically pumped laser diodes based on solution‐processed semiconductors is a long‐standing challenge. Metal halide perovskites have shown great potential toward this goal due to their excellent optoelectronic properties. Continuous‐wave (CW) optically pumped lasing in a real electroluminescent device represents a key step to current‐injection laser diodes, but it has not yet been realized. This is mainly due to the challenge of incorporating a resonant cavity into an efficient light‐emitting diode (LED) able to sustain intensive carrier injection. Here, CW lasing is reported in an efficient perovskite LED with an integrated distributed feedback resonator, which shows a low lasing threshold of 220 W cm −2 at 110 K. Importantly, the LED works well at a current density of 330 A cm −2 , indicating the carrier injection rate already exceeds the threshold of optically pumping. The results suggest that electrically pumped perovskite laser diodes can be achieved once the Joule heating issue is overcome.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Organic Light-Emitting Diodes Research · Solid State Laser Technologies

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Key Laboratory of Flexible Electronics (KLOFE) Institute of Advanced Materials (IAM) & School of Flexible Electronics (Future Technologies) Nanjing Tech University (NanjingTech) 30 South Puzhu Road Nanjing 211816 China

Strait Laboratory of Flexible Electronics (SLoFE) Fuzhou 350117 China

Strait Institute of Flexible Electronics (SIFE Future Technologies) Fujian Normal University Fuzhou 350117 China

Institute of Joint Key Laboratory of the Applied Physics and Materials Engineering University of Macao Avenida da Universidade Taipa Macao 999078 China

Changzhou University 21 Middle Gehu Road Changzhou 213164 China

Funding

National Natural Science Foundation of China · Synergetic Innovation Center for Organic Electronics and Information Displays

References (33)

Show source-provided references
1. 10.1364/OE.19.00817910.1364/OE.19.008179 ↗
2. 10.1364/OE.25.03291910.1364/OE.25.032919 ↗
3. 10.1002/adom.20190037710.1002/adom.201900377 ↗
4. 10.1038/s41566-021-00827-610.1038/s41566-021-00827-6 ↗
5. 10.1002/adma.20220777710.1002/adma.202207777 ↗
6. 10.1021/acs.chemrev.6b0013610.1021/acs.chemrev.6b00136 ↗
7. 10.1038/nphoton.2016.6210.1038/nphoton.2016.62 ↗
8. 10.1038/s41586-018-0576-210.1038/s41586-018-0576-2 ↗
9. 10.1038/s41467-018-03049-710.1038/s41467-018-03049-7 ↗
10. 10.1038/s41563-020-0784-710.1038/s41563-020-0784-7 ↗
11. 10.1021/acs.nanolett.0c0359310.1021/acs.nanolett.0c03593 ↗
12. 10.1038/s41566-017-0047-610.1038/s41566-017-0047-6 ↗
13. 10.1021/acsnano.8b0485410.1021/acsnano.8b04854 ↗
14. 10.1038/s41586-020-2621-110.1038/s41586-020-2621-1 ↗
15. 10.1002/adom.20200198210.1002/adom.202001982 ↗
16. 10.1002/adma.20200075210.1002/adma.202000752 ↗
17. 10.1038/s41467-018-07383-810.1038/s41467-018-07383-8 ↗
18. 10.1002/adma.20210486710.1002/adma.202104867 ↗
19. 10.1002/adom.20190129710.1002/adom.201901297 ↗
20. 10.1021/acsphotonics.8b0141310.1021/acsphotonics.8b01413 ↗
21. 10.1021/acs.nanolett.6b0194610.1021/acs.nanolett.6b01946 ↗
22. 10.1002/lpor.20220018910.1002/lpor.202200189 ↗
23. 10.1002/adom.20170098210.1002/adom.201700982 ↗
24. 10.1039/C9RA07442B10.1039/C9RA07442B ↗
25. 10.1021/acs.jpclett.9b0065810.1021/acs.jpclett.9b00658 ↗
26. 10.1021/acs.nanolett.0c0246210.1021/acs.nanolett.0c02462 ↗
27. 10.1002/adma.20200681910.1002/adma.202006819 ↗
28. 10.1021/acsphotonics.2c0007110.1021/acsphotonics.2c00071 ↗
29. 10.1063/5.005245810.1063/5.0052458 ↗
30. 10.1038/nphoton.2009.17310.1038/nphoton.2009.173 ↗
31. 10.1038/s41467-019-08929-010.1038/s41467-019-08929-0 ↗
32. 10.1039/D2MH01382G10.1039/D2MH01382G ↗
33. 10.1063/1.363869910.1063/1.3638699 ↗