journal article·2023-03Open access

Optically Excited Lasing in a Cavity‐Based, High‐Current‐Density Quantum Dot Electroluminescent Device

Namyoung Ahn, Young‐Shin Park, Clément Livache, Jun Du, Kivanc Gungor, Jaehoon Kim, Victor I. Klimov

Advanced Materials· Volume 35· Issue 9

Abstract

Abstract Laser diodes based on solution‐processable materials can benefit numerous technologies including integrated electronics and photonics, telecommunications, and medical diagnostics. An attractive system for implementing these devices is colloidal semiconductor quantum dots (QDs). The progress towards a QD laser diode has been hampered by rapid nonradiative Auger decay of optical‐gain‐active multicarrier states, fast device degradation at high current densities required for laser action, and unfavorable competition between optical gain and optical losses in a multicomponent device stack. Here we resolve some of these challenges and demonstrate optically excited lasing from fully functional high‐current density electroluminescent (EL) devices with an integrated optical resonator. This advance has become possible due to excellent optical gain properties of continuously graded QDs and a refined device architecture, which allows for highly efficient light amplification in a thin, EL‐active QD layer.
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Research context

OpenAlex topics: Quantum Dots Synthesis And Properties · Molecular Junctions and Nanostructures · Semiconductor Quantum Structures and Devices

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Nanotechnology and Advanced Spectroscopy Team C‐PCS Chemistry Division Los Alamos National Laboratory Los Alamos NM 87545 USA

State Key Laboratory of Molecular Reaction Dynamics Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian Liaoning 116023 China

Funding

Los Alamos National Laboratory

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