journal article·2018-05

Controlled Homoepitaxial Growth of Hybrid Perovskites

Yusheng Lei, Yimu Chen, Yue Gu, Chunfeng Wang, Zhenlong Huang, Haoliang Qian, Jiuyuan Nie, Geoff Hollett, Woojin Choi, Yugang Yu, NamHeon Kim, Chonghe Wang, Tianjiao Zhang, Hongjie Hu, Yunxi Zhang, Xiaoshi Li, Yang Li, Wanjun Shi, Zhaowei Liu, Michael J. Sailor, Lin Dong, Yu‐Hwa Lo, Jian Luo, Sheng Xu

Advanced Materials· Volume 30· Issue 20
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Abstract

Abstract Organic–inorganic hybrid perovskites have demonstrated tremendous potential for the next‐generation electronic and optoelectronic devices due to their remarkable carrier dynamics. Current studies are focusing on polycrystals, since controlled growth of device compatible single crystals is extremely challenging. Here, the first chemical epitaxial growth of single crystal CH3NH3PbBr3 with controlled locations, morphologies, and orientations, using combined strategies of advanced microfabrication, homoepitaxy, and low temperature solution method is reported. The growth is found to follow a layer‐by‐layer model. A light emitting diode array, with each CH3NH3PbBr3 crystal as a single pixel, with enhanced quantum efficiencies than its polycrystalline counterparts is demonstrated.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Magnetic and transport properties of perovskites and related materials · Electronic and Structural Properties of Oxides

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Nanoengineering University of California San Diego La Jolla CA 92093 USA

Materials Science and Engineering Program University of California San Diego La Jolla CA 92093 USA

The Key Laboratory of Materials Processing and Mold of Ministry of Education School of Materials Science and Engineering Zhengzhou University Zhengzhou Henan 450001 P. R. China

School of Microelectronics and Solid State Electronics University of Electronic Science and Technology of China Chengdu Sichuan 611731 P. R. China

Department of Electrical and Computer Engineering University of California San Diego La Jolla CA 92093 USA

Zhejiang Research Institute of Chemical Industry Hangzhou Zhejiang 310023 P. R. China

Department of Chemistry and Biochemistry University of California San Diego La Jolla CA 92093 USA

Funding

National Science Foundation

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