journal article·2025-01

Rational Engineering of Phase‐Pure 2D Perovskite Solar Cells

Ke Guo, Wenzhen Lv, He Wang, Mingguang Li, Ligang Xu, Runfeng Chen, Guichuan Xing, Guangbao Wu

Advanced Functional Materials· Volume 35· Issue 2
Publisher page

Abstract

Abstract 2D perovskite structures have gained significant attention due to their reliable long‐term stability. Unlike quasi‐2D perovskites, phase‐pure 2D perovskites exhibit a flattened energy landscape and low energy transfer losses, offering substantial benefits for enhancing device efficiency and stability. Recent research on phase‐pure 2D perovskites has shown significant progress, attributed to their unique properties. This review delineates advancements in the study of phase‐pure 2D perovskite materials and elucidates the relationships between crystal structure design, growth, and device performance regulation. Additionally, it summarizes techniques for characterizing phase‐pure 2D structures and methods for their precise synthesis. Finally, an outlook on the future development of phase‐pure 2D perovskites, highlighting the scientific and technological challenges in current research is provided.
Source: crossref · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Conducting polymers and applications · Chalcogenide Semiconductor Thin Films

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

State Key Laboratory of Organic Electronics and Information Displays and Institute of Advanced Materials (IAM) Nanjing University of Posts and Telecommunications 9 Wenyuan Road Nanjing 210023 P. R. China

Joint Key Laboratory of the Ministry of Education Institute of Applied Physics and Materials Engineering University of Macau Avenida da Universidade, Taipa Macau 999078 P. R. China

Funding

National Natural Science Foundation of China · Science and Technology Development Fund

References (100+)

Show source-provided references
1. 10.1039/C5EE03255E10.1039/C5EE03255E ↗
2. 10.1126/science.adm947410.1126/science.adm9474 ↗
3. National Renewable Energy Laboratory B.R‐C.E. Chart www.nrel.gov/ncpv/images/efficiency_chart.jpg.
4. 10.1038/s41586-024-07723-310.1038/s41586-024-07723-3 ↗
5. 10.1002/adma.20240085210.1002/adma.202400852 ↗
6. 10.1038/s41578-023-00582-w10.1038/s41578-023-00582-w ↗
7. 10.1038/s41560-024-01487-w10.1038/s41560-024-01487-w ↗
8. 10.1038/s41467-018-07382-910.1038/s41467-018-07382-9 ↗
9. Chen Y. · Adv. Mater. · 2018 · 30
10. 10.1007/BF0150752710.1007/BF01507527 ↗
11. 10.1021/jacs.5b1174010.1021/jacs.5b11740 ↗
12. 10.1016/j.chempr.2019.07.02410.1016/j.chempr.2019.07.024 ↗
13. 10.1002/aenm.20170097910.1002/aenm.201700979 ↗
14. 10.1039/b403482a10.1039/b403482a ↗
15. 10.1021/ja00006a07610.1021/ja00006a076 ↗
16. 10.1021/jacs.5b0379610.1021/jacs.5b03796 ↗
17. 10.1002/advs.20200184310.1002/advs.202001843 ↗
18. 10.1021/jacs.3c0979310.1021/jacs.3c09793 ↗
19. 10.1038/s41467-020-15451-110.1038/s41467-020-15451-1 ↗
20. 10.1002/adma.20210584910.1002/adma.202105849 ↗
21. 10.1016/j.mtnano.2021.10011710.1016/j.mtnano.2021.100117 ↗
22. 10.1002/adfm.20220528910.1002/adfm.202205289 ↗
23. 10.1002/advs.20210484810.1002/advs.202104848 ↗
24. 10.1021/jacs.0c0386010.1021/jacs.0c03860 ↗
25. 10.1021/acs.chemrev.3c0021410.1021/acs.chemrev.3c00214 ↗
26. 10.1002/adma.20200147010.1002/adma.202001470 ↗
27. 10.1021/acs.chemmater.9b0131810.1021/acs.chemmater.9b01318 ↗
28. 10.1039/C6EE03014A10.1039/C6EE03014A ↗
29. 10.1126/science.aay704410.1126/science.aay7044 ↗
30. 10.1126/science.abj118610.1126/science.abj1186 ↗
31. 10.1021/acsnano.0c0982210.1021/acsnano.0c09822 ↗
32. 10.1016/j.chempr.2021.04.00210.1016/j.chempr.2021.04.002 ↗
33. 10.1002/anie.20200521110.1002/anie.202005211 ↗
34. 10.1021/jacs.3c1357610.1021/jacs.3c13576 ↗
35. 10.1038/s41586-024-07189-310.1038/s41586-024-07189-3 ↗
36. 10.1038/s41467-023-43016-510.1038/s41467-023-43016-5 ↗
37. 10.1021/acs.chemrev.0c0100610.1021/acs.chemrev.0c01006 ↗
38. 10.1021/jacs.8b1085110.1021/jacs.8b10851 ↗
39. 10.1016/j.nantod.2022.10139410.1016/j.nantod.2022.101394 ↗
40. 10.1002/aenm.20210297310.1002/aenm.202102973 ↗
41. 10.1021/jacs.7b1255110.1021/jacs.7b12551 ↗
42. 10.1016/j.matt.2020.11.01110.1016/j.matt.2020.11.011 ↗
43. 10.1002/aenm.20170016210.1002/aenm.201700162 ↗
44. 10.1039/D0SC04144K10.1039/D0SC04144K ↗
45. 10.1021/acsnano.9b0443710.1021/acsnano.9b04437 ↗
46. 10.1016/j.joule.2023.03.01010.1016/j.joule.2023.03.010 ↗
47. 10.1007/s40820-023-01141-210.1007/s40820-023-01141-2 ↗
48. 10.1038/s42005-018-0082-810.1038/s42005-018-0082-8 ↗
49. 10.1021/acs.nanolett.3c0388710.1021/acs.nanolett.3c03887 ↗
50. 10.1093/nsr/nwab11110.1093/nsr/nwab111 ↗
51. 10.1021/jacs.0c0336310.1021/jacs.0c03363 ↗
52. 10.1021/jacs.3c0860410.1021/jacs.3c08604 ↗
53. 10.1002/adma.20221212610.1002/adma.202212126 ↗
54. 10.1002/adma.20210508310.1002/adma.202105083 ↗
55. 10.1021/acsenergylett.9b0089210.1021/acsenergylett.9b00892 ↗
56. Zhang H. · Angew. Chem., Int. Ed. · 2024 · 63
57. 10.1002/adma.20230742210.1002/adma.202307422 ↗
58. 10.1038/s41586-024-07764-810.1038/s41586-024-07764-8 ↗
59. 10.1021/jacs.9b0284610.1021/jacs.9b02846 ↗
60. 10.1073/pnas.181100611510.1073/pnas.1811006115 ↗
61. 10.1021/jacs.9b0132710.1021/jacs.9b01327 ↗
62. 10.1021/jacs.8b0771210.1021/jacs.8b07712 ↗
63. 10.1021/jacs.8b0054210.1021/jacs.8b00542 ↗
64. 10.1021/acs.inorgchem.7b0109410.1021/acs.inorgchem.7b01094 ↗
65. 10.1002/anie.20140646610.1002/anie.201406466 ↗
66. 10.1021/acsami.1c1586010.1021/acsami.1c15860 ↗
67. 10.1021/jacs.1c0368710.1021/jacs.1c03687 ↗
68. 10.1002/aenm.20190405010.1002/aenm.201904050 ↗
69. 10.1021/jacs.9b0639810.1021/jacs.9b06398 ↗
70. 10.1126/science.aal421110.1126/science.aal4211 ↗
71. 10.1016/j.xcrp.2021.10060110.1016/j.xcrp.2021.100601 ↗
72. 10.1038/s44160-023-00422-310.1038/s44160-023-00422-3 ↗
73. 10.1021/jacs.0c1132810.1021/jacs.0c11328 ↗
74. 10.1038/s41578-023-00560-210.1038/s41578-023-00560-2 ↗
75. 10.1038/s41467-019-08980-x10.1038/s41467-019-08980-x ↗
76. 10.1038/s41566-022-00985-110.1038/s41566-022-00985-1 ↗
77. 10.1021/acsenergylett.7b0124510.1021/acsenergylett.7b01245 ↗
78. 10.1007/s40843-018-9294-510.1007/s40843-018-9294-5 ↗
79. 10.1021/acsnano.6b0153510.1021/acsnano.6b01535 ↗
80. 10.1038/nature1830610.1038/nature18306 ↗
81. 10.1002/smll.20220678710.1002/smll.202206787 ↗
82. 10.1021/acs.nanolett.0c0391410.1021/acs.nanolett.0c03914 ↗
83. 10.1002/adma.20180199610.1002/adma.201801996 ↗
84. 10.1021/acsenergylett.3c0261610.1021/acsenergylett.3c02616 ↗
85. 10.1038/s41563-018-0154-x10.1038/s41563-018-0154-x ↗
86. 10.1021/ja01167a00110.1021/ja01167a001 ↗
87. 10.1021/acs.chemrev.0c0045410.1021/acs.chemrev.0c00454 ↗
88. 10.1016/j.pmatsci.2021.10082110.1016/j.pmatsci.2021.100821 ↗
89. 10.1002/smll.20100202210.1002/smll.201002022 ↗
90. 10.1039/C9CS00711C10.1039/C9CS00711C ↗
91. 10.1038/s41467-021-22049-810.1038/s41467-021-22049-8 ↗
92. 10.1039/D2MH01408D10.1039/D2MH01408D ↗
93. 10.1038/nmat401410.1038/nmat4014 ↗
94. 10.1016/j.joule.2019.09.02010.1016/j.joule.2019.09.020 ↗
95. 10.1126/science.aaf806010.1126/science.aaf8060 ↗
96. 10.1002/anie.20191418310.1002/anie.201914183 ↗
97. 10.1126/science.abq765210.1126/science.abq7652 ↗
98. 10.1002/adma.20200717610.1002/adma.202007176 ↗
99. 10.1038/s41560-020-00721-510.1038/s41560-020-00721-5 ↗
100. 10.1002/cey2.25110.1002/cey2.251 ↗