Chiral Perovskite Nanowire Optoelectronic Synapse for Full‐Stokes Polarization‐Resolved Perception and Reservoir Computing

Abstract Full‐Stokes polarization‐resolved photonic artificial synapse (PAS) devices with in‐sensor computing capabilities show great potential for multimode vision perception and processing. However, current polarization‐resolved PAS devices are limited to monotonic recognition of linearly polarized light or circularly polarized light. Here, the study develops a chiral perovskite nanowire‐based PAS device as a full‐Stokes polarimeter to achieve polarization‐dependent neuromorphic optoelectronics. The device demonstrates a significantly high circular dichroism of over 400 millidegree and intrinsic linear dichroism, contributing to effectively sensing polarized light. Efficient charge separation at the perovskite NW/MXene heterostructure results in a prolonged carrier lifetime, thereby achieving a high responsivity of 2.3 AW⁻¹, excellent synaptic behavior, and low power consumption of 0.5 pJ per synaptic stimuli. Significantly, the polarization‐modulated reservoir computing is developed based on the full‐Stokes PAS device, which exhibits a low normalized root mean square error of 0.023 in the chaotic system forecasting task. The single‐nanowire PAS device with the capability of sensing full‐Stokes parameters demonstrates great significance in building advanced energy‐efficient polarization‐resolved nanoscale neuromorphic vision systems.