Charge State Manipulation of NV Centers in Diamond under Phonon-Assisted Anti-Stokes Excitation of NV0
Source abstract
Abstract
The manipulation of the charge states of nitrogen-vacancy (NV) centers in diamond is a prerequisite for next-generation quantum sensing, communication, and computing. Here, we use phonon-assisted anti-Stokes excitation to realize the reversible conversion between the NV0 and NV– states. In this case, we observe two decay processes of NV– centers with lifetimes as long as tens of seconds. By studying the kinetics of spectral structure evolution of NV– states, we find that the spectral structure of the NV– center is modulated by the charge state transition process under anti-Stokes excitation. We propose that the main reason is the local electric field generated by the ionization of the NV–, which changes the radiation environment of the color centers. Our results might provide an alternative method to control the charge states of nitrogen-vacancy centers.
Source: openalex_inverted_index · Quality: baseline
Research context
OpenAlex topics: Diamond and Carbon-based Materials Research · High-pressure geophysics and materials · Advanced Fiber Laser Technologies
SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.
Affiliations
State Key Laboratory of Superlattices and Microstructures, Institute of Semiconductors, & Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Chinese Academy of Sciences, Beijing 100083, People’s Republic of China
Beijing Academy of Quantum Information Sciences, Beijing 100193, People’s Republic of China
Henan Key Laboratory of Diamond Optoelectronic Materials and Devices, Key Laboratory of Material Physics, Ministry of Education, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou 450052, People’s Republic of China
Funding
Ministry of Science and Technology of the People's Republic of China · National Natural Science Foundation of China · Chinese Academy of Sciences
References (54)
Show source-provided references
1. 10.1126/sciadv.160242910.1126/sciadv.1602429 ↗
2. 10.1126/science.aao029010.1126/science.aao0290 ↗
3. 10.1103/PhysRevApplied.13.04402310.1103/PhysRevApplied.13.044023 ↗
4. 10.1038/nmat242010.1038/nmat2420 ↗
5. 10.1103/PhysRevLett.93.13050110.1103/PhysRevLett.93.130501 ↗
6. 10.1103/PhysRevLett.117.01550210.1103/PhysRevLett.117.015502 ↗
7. 10.1103/PhysRevA.95.02233810.1103/PhysRevA.95.022338 ↗
8. 10.1016/j.carbon.2018.10.08410.1016/j.carbon.2018.10.084 ↗
9. 10.1063/1.486812810.1063/1.4868128 ↗
10. 10.1063/1.489297110.1063/1.4892971 ↗
11. 10.1039/C6NR07834F10.1039/C6NR07834F ↗
12. 10.1103/PhysRevB.80.11520210.1103/PhysRevB.80.115202 ↗
13. 10.1007/s10812-015-0092-110.1007/s10812-015-0092-1 ↗
14. 10.1021/ja063303n10.1021/ja063303n ↗
15. 10.1063/1.357376810.1063/1.3573768 ↗
16. 10.1103/PhysRevB.83.08130410.1103/PhysRevB.83.081304 ↗
17. 10.1063/1.480187110.1063/1.4801871 ↗
18. 10.1038/ncomms172910.1038/ncomms1729 ↗
19. 10.1088/1367-2630/15/1/01306410.1088/1367-2630/15/1/013064 ↗
20. 10.1021/nl501927y10.1021/nl501927y ↗
21. 10.1021/acs.nanolett.6b0502310.1021/acs.nanolett.6b05023 ↗
22. 10.1103/PhysRevLett.109.09740410.1103/PhysRevLett.109.097404 ↗
23. 10.1021/nl102156m10.1021/nl102156m ↗
24. 10.1103/PhysRevB.94.02410110.1103/PhysRevB.94.024101 ↗
25. 10.1038/nature1172110.1038/nature11721 ↗
26. 10.1021/acs.jpclett.8b0286210.1021/acs.jpclett.8b02862 ↗
27. 10.1038/nphoton.2016.12210.1038/nphoton.2016.122 ↗
28. 10.1038/nphoton.2014.8410.1038/nphoton.2014.84 ↗
29. 10.1073/pnas.050828210210.1073/pnas.0508282102 ↗
30. 10.1038/s41578-018-0008-910.1038/s41578-018-0008-9 ↗
31. 10.1038/nphoton.2010.17410.1038/nphoton.2010.174 ↗
32. 10.1103/RevModPhys.84.77710.1103/RevModPhys.84.777 ↗
33. 10.1088/0953-8984/18/21/S0910.1088/0953-8984/18/21/S09 ↗
34. 10.1038/s41467-019-13332-w10.1038/s41467-019-13332-w ↗
35. 10.1126/science.aax940610.1126/science.aax9406 ↗
36. 10.1103/PhysRevLett.97.08300210.1103/PhysRevLett.97.083002 ↗
37. Tran T. T. · Appl. Phys. Lett. · 2019 · 115 · 07110110.1063/1.5109234 ↗
38. 10.1038/s41467-021-23471-810.1038/s41467-021-23471-8 ↗
39. 10.1103/PhysRevLett.106.15760110.1103/PhysRevLett.106.157601 ↗
40. 10.1103/PhysRevB.51.1668110.1103/PhysRevB.51.16681 ↗
41. 10.1021/acs.nanolett.8b0173910.1021/acs.nanolett.8b01739 ↗
42. 10.7498/aps.69.2020039510.7498/aps.69.20200395 ↗
43. 10.1038/159096b010.1038/159096b0 ↗
44. 10.1126/sciadv.abm591210.1126/sciadv.abm5912 ↗
45. 10.1103/PhysRevA.97.06340810.1103/PhysRevA.97.063408 ↗
46. 10.1103/PhysRevLett.120.11740110.1103/PhysRevLett.120.117401 ↗
47. Maze J. R. · New J. Phys. · 2011 · 13 · 780
48. 10.1021/nl504941q10.1021/nl504941q ↗
49. 10.1103/PhysRevLett.110.02740110.1103/PhysRevLett.110.027401 ↗
50. 10.1021/acsphotonics.0c0112310.1021/acsphotonics.0c01123 ↗
51. 10.1038/s41467-017-01993-410.1038/s41467-017-01993-4 ↗
52. 10.1038/s41467-020-16330-510.1038/s41467-020-16330-5 ↗
53. 10.1038/nature1056210.1038/nature10562 ↗
54. 10.1103/PhysRevB.95.23530610.1103/PhysRevB.95.235306 ↗