journal article·2022-03-16Open access

Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities

Jérôme Gautier, Minghao Li, Thomas W. Ebbesen, Cyriaque Genet

ACS Photonics· Volume 9· Issue 3

Abstract

We design, in a most simple way, Fabry-Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin-orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry.
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Research context

OpenAlex topics: Strong Light-Matter Interactions · Plasmonic and Surface Plasmon Research · Quantum and electron transport phenomena

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Affiliations

Université de Strasbourg, CNRS, Institut de Science et d’Ingénierie Supramoléculaires, UMR 7006, F-67000 Strasbourg, France

Funding

Agence Nationale de la Recherche · Institut National de la Sant? et de la Recherche M?dicale · Universit? de Strasbourg · Centre National de la Recherche Scientifique · H2020 European Research Council

References (37)

Show source-provided references
1. 10.1364/OE.16.01255910.1364/OE.16.012559 ↗
2. 10.1103/PhysRevLett.124.03320110.1103/PhysRevLett.124.033201 ↗
3. 10.1021/acs.accounts.9b0046010.1021/acs.accounts.9b00460 ↗
4. 10.1103/PhysRevLett.114.20300310.1103/PhysRevLett.114.203003 ↗
5. 10.1021/acsphotonics.7b0103210.1021/acsphotonics.7b01032 ↗
6. 10.1364/OME.9.00053610.1364/OME.9.000536 ↗
7. 10.1038/nature2103710.1038/nature21037 ↗
8. 10.1038/s41563-020-00801-710.1038/s41563-020-00801-7 ↗
9. 10.1021/acs.accounts.6b0029510.1021/acs.accounts.6b00295 ↗
10. 10.1103/PhysRevX.10.04104310.1103/PhysRevX.10.041043 ↗
11. 10.1103/PhysRevA.86.01384510.1103/PhysRevA.86.013845 ↗
12. 10.1038/nphoton.2015.20110.1038/nphoton.2015.201 ↗
13. Kastler A. · C. R. Acad. Sci. B · 1970 · 271 · 999
14. 10.1038/nature1368010.1038/nature13680 ↗
15. 10.1364/AO.39.00064210.1364/AO.39.000642 ↗
16. 10.1063/1.492196910.1063/1.4921969 ↗
17. 10.1063/5.002500610.1063/5.0025006 ↗
18. 10.1103/PhysRevLett.97.16740110.1103/PhysRevLett.97.167401 ↗
19. 10.1088/1464-4258/11/7/07400910.1088/1464-4258/11/7/074009 ↗
20. 10.1364/OL.38.00113410.1364/OL.38.001134 ↗
21. Li, M. Polarimétrie de Mueller pour sonder les chiralités moléculaires et optiques. Ph.D. thesis, Université de Strasbourg, 2020.
22. 10.1016/0009-2614(94)87122-110.1016/0009-2614(94)87122-1 ↗
23. Drezet A. · 201410.1201/b17632-3 ↗
24. 10.1021/acsphotonics.7b0066610.1021/acsphotonics.7b00666 ↗
25. 10.1021/nl801794d10.1021/nl801794d ↗
26. 10.1038/srep0744210.1038/srep07442 ↗
27. 10.1021/nl300316f10.1021/nl300316f ↗
28. 10.1002/anie.19890021110.1002/anie.198900211 ↗
29. 10.1002/ijch.19760000210.1002/ijch.197600002 ↗
30. 10.1016/S0040-4039(01)81302-210.1016/S0040-4039(01)81302-2 ↗
31. 10.1364/OL.35.00055910.1364/OL.35.000559 ↗
32. Lakhtakia A. · 1989 · 335
33. Lindell I. V. · 1994
34. 10.1021/acsphotonics.6b0020110.1021/acsphotonics.6b00201 ↗
35. 10.3390/sym1109111310.3390/sym11091113 ↗
36. Anatoly S. · 2001
37. 10.1088/2040-8978/18/8/08560110.1088/2040-8978/18/8/085601 ↗