journal article·2025-11-25

Quantum-Geometry–Enabled Terahertz Rectification in the Weyl Semimetal TaP

Wenqi Mo, Xuyang Lv, Bojin Zhao, Libo Zhang, Yunduo Zhang, Kening Xiao, Yichong Zhang, Yiran Tan, Zongju Huo, Bolang Peng, Yuanfeng Wen, Shijian Tian, Shi Zhang, Mengjie Jiang, Kaixuan Zhang, Bangjian Zhao, Hailong Qiu, Lin Wang, Xiaoshuang Chen

ACS Nano· Volume 19· Issue 46
Publisher page

Abstract

Noncentrosymmetric crystals can rectify light into a direct current (DC) through the second-order nonlinear response governed by the Berry-curvature dipole (BCD), an effect that becomes particularly efficient for low-energy terahertz (THz) photons. Topological Weyl semimetals (WSMs), with their large Berry curvature near the Weyl points and intrinsically broken inversion symmetry, represent an ideal platform to realize this effect. However, directly experimentally demonstrating a BCD-driven photoresponse in the THz regime remains a significant challenge. Here, we demonstrate room-temperature, junction-free terahertz current rectification in type-I Weyl semimetal tantalum phosphide (TaP) explicitly driven by its intrinsic Berry curvature dipole. We observe that transverse THz polarization generates longitudinal photocurrents with a fast response time (0.96 μs) across a broad bandwidth (0.04-0.53 THz), directly confirming BCD-imposed momentum-space asymmetry and its topological origin. Operating as a room-temperature heterodyne mixer, the TaP device achieves a remarkable 25 dB conversion gain over a 20 GHz instantaneous intermediate-frequency (IF) bandwidth. These results establish Weyl semimetals as a paradigm for topological optoelectronics, where a deeper understanding of quantum geometric effects directly enables the development of high-performance terahertz devices for applications such as 6G wireless communication.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Topological Materials and Phenomena · Metamaterials and Metasurfaces Applications · Graphene research and applications

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

College of Physics and Optoelectronic Engineering, Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, No. 1, Sub-Lane Xiangshan, Xihu, Hangzhou 310024, China

State Key Laboratory for Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, 500 Yu-Tian Road, Shanghai 200083, China

State Key Laboratory of Crystal Materials, Tianjin Key Laboratory of Functional Crystal Materials, Institute of Functional Crystals

Tianjin University of Technology

CAS Key Laboratory of Nanophotonic Materials and Devices & Key Laboratory of Nanodevices and Applications, i-Lab, Suzhou Institute of Nano-Tech and Nano-Bionics

Chinese Academy of Sciences

Funding

Natural Science Foundation of Shanghai Municipality · National Key Research and Development Program of China · National Natural Science Foundation of China · National Outstanding Youth Foundation of China · Chinese Academy of Sciences · National Key Laboratory of Infrared Detection Technologies · State Key Laboratory of Photonics and Communications, Peking University

References (34)

Show source-provided references
1. 10.1126/sciadv.150152410.1126/sciadv.1501524 ↗
2. 10.1126/sciadv.abj107610.1126/sciadv.abj1076 ↗
3. 10.1038/s41467-024-47643-410.1038/s41467-024-47643-4 ↗
4. 10.1038/nphoton.2015.24910.1038/nphoton.2015.249 ↗
5. 10.1038/s41565-020-00839-310.1038/s41565-020-00839-3 ↗
6. 10.1016/j.infrared.2025.10589610.1016/j.infrared.2025.105896 ↗
7. 10.1038/s41586-021-04105-x10.1038/s41586-021-04105-x ↗
8. 10.1038/s41578-021-00301-310.1038/s41578-021-00301-3 ↗
9. 10.1038/s41563-019-0297-410.1038/s41563-019-0297-4 ↗
10. 10.48550/arXiv.1712.0495110.48550/arXiv.1712.04951 ↗
11. 10.1038/s41563-019-0296-510.1038/s41563-019-0296-5 ↗
12. 10.1021/ja00049a02910.1021/ja00049a029 ↗
13. 10.1038/nphoton.2016.20910.1038/nphoton.2016.209 ↗
14. 10.1126/science.124225310.1126/science.1242253 ↗
15. 10.1088/0022-3727/47/37/37400110.1088/0022-3727/47/37/374001 ↗
16. 10.1038/nmat341710.1038/nmat3417 ↗
17. 10.1126/sciadv.adt000610.1126/sciadv.adt0006 ↗
18. 10.1126/sciadv.adv076810.1126/sciadv.adv0768 ↗
19. 10.1126/sciadv.abi839810.1126/sciadv.abi8398 ↗
20. 10.1038/srep4666410.1038/srep46664 ↗
21. 10.1038/s41928-025-01397-z10.1038/s41928-025-01397-z ↗
22. 10.1103/PhysRevB.107.12510610.1103/PhysRevB.107.125106 ↗
23. 10.1038/ncomms1161510.1038/ncomms11615 ↗
24. 10.1038/ncomms837310.1038/ncomms8373 ↗
25. 10.1126/science.aaa929710.1126/science.aaa9297 ↗
26. 10.1126/sciadv.150109210.1126/sciadv.1501092 ↗
27. 10.1038/s41563-019-0320-910.1038/s41563-019-0320-9 ↗
28. 10.1038/nphys396910.1038/nphys3969 ↗
29. 10.1103/PhysRevLett.115.21680610.1103/PhysRevLett.115.216806 ↗
30. 10.1021/acsnano.4c1737110.1021/acsnano.4c17371 ↗
31. 10.1103/PhysRevLett.115.21680610.1103/PhysRevLett.115.216806 ↗
32. 10.1126/sciadv.adq064210.1126/sciadv.adq0642 ↗
33. 10.1021/acsaelm.3c0151110.1021/acsaelm.3c01511 ↗
34. 10.1021/acs.nanolett.8b0057410.1021/acs.nanolett.8b00574 ↗