journal article·2020-04-28

Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics

Chun Ma, Sarah Clark, Zhixiong Liu, Liangliang Liang, Yuliar Firdaus, Ran Tao, Ali Han, Xiaogang Liu, Lain-Jong Li, Thomas D. Anthopoulos, Mark C. Hersam, Tom Wu

ACS Nano· Volume 14· Issue 4
Publisher page

Abstract

Benefiting from their extraordinary physical properties, methylammonium lead halide perovskites (PVKs) have attracted significant attention in optoelectronics. However, the PVK-based devices suffer from low carrier mobility and high operation voltage. Here, we utilize sorted semiconducting single-walled carbon nanotubes (95% s-SWCNTs) to enhance the performance of thin-film transistors (TFTs) based on the mixed-cation perovskite (MA1–xFAx)Pb(I1–xBrx)3, enabling mixed-dimensional solution-processed electronics with high mobility (32.25 cm2/(V s)) and low voltage (∼3 V) operation. The resulting mixed-dimensional PVK/SWCNT TFTs possess ON/OFF ratios on the order of 107, enabling the fabrication of high-gain inverters.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · Conducting polymers and applications · ZnO doping and properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

King Abdullah University of Science and Technology (Kaust), Kaust Solar Center, Thuwal 23955-6900, Saudi Arabia

Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, United States

Department of Chemistry, National University of Singapore, Singapore, 119077, Singapore

Department of Chemistry, Department of Electrical and Computer Engineering, Northwestern University, Evanston, Illinois 60208, United States

School of Materials Science and Engineering, University of New South Wales (UNSW), Sydney, NSW 2052, Australia

Funding

King Abdullah University of Science and Technology · Division of Materials Research

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