journal article·2025-07-01

Quantum Sensing with Spin Defects Beyond Diamond

Henry Roberts, Hamza Abudayyeh, Xiaoqin Li, Xiuling Li

ACS Nano· Volume 19· Issue 25
Publisher page

Abstract

Spin defects in solid-state materials offer a platform for quantum sensing that combines the properties of atom-like systems with the scalability, versatility, and technological maturity of semiconductor devices. The past decade has seen increasing interest in host materials beyond diamond which can offer additional functionality and more effectively leverage the advantage of the existing semiconductor ecosystem. This review provides a survey and comparison of spin defects in silicon carbide, hexagonal boron nitride, and gallium nitride with an emphasis on their applications to magnetometry, electrometry, thermometry, and strain sensing. A practical overview of quantum sensing protocols and sensitivity enhancement is provided along with a final discussion of the future direction of the field and remaining challenges.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Diamond and Carbon-based Materials Research · Semiconductor materials and devices · Metal and Thin Film Mechanics

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Department of Electrical and Computer Engineering and Microelectronics Research Center

University of Texas at Austin

Texas Quantum Institute

Department of Physics and Center for Complex Quantum Systems

Funding

Welch Foundation · National Science Foundation · Texas Quantum Institute

References (100+)

Show source-provided references
1. 10.26636/jtit.2010.1.101510.26636/jtit.2010.1.1015 ↗
2. 10.1109/6.59166410.1109/6.591664 ↗
3. 10.1103/PhysRevLett.1.36810.1103/PhysRevLett.1.368 ↗
4. 10.1038/3015610.1038/30156 ↗
5. 10.1098/rspa.1976.003910.1098/rspa.1976.0039 ↗
6. 10.1103/PhysRevLett.67.342010.1103/PhysRevLett.67.3420 ↗
7. 10.1016/j.physrep.2013.02.00110.1016/j.physrep.2013.02.001 ↗
8. 10.1126/science.276.5321.201210.1126/science.276.5321.2012 ↗
9. 10.1016/j.physrep.2013.02.00110.1016/j.physrep.2013.02.001 ↗
10. 10.1038/s41566-018-0232-210.1038/s41566-018-0232-2 ↗
11. 10.1038/s41578-021-00306-y10.1038/s41578-021-00306-y ↗
12. 10.1002/elt2.7010.1002/elt2.70 ↗
13. 10.1039/D1RA00397F10.1039/D1RA00397F ↗
14. 10.1557/mrs.2014.9610.1557/mrs.2014.96 ↗
15. 10.1080/26941112.2021.195628710.1080/26941112.2021.1956287 ↗
16. 10.1103/RevModPhys.89.03500210.1103/RevModPhys.89.035002 ↗
17. 10.1103/RevModPhys.92.01500410.1103/RevModPhys.92.015004 ↗
18. 10.3390/s2116556810.3390/s21165568 ↗
19. 10.1088/0268-1242/26/6/06400610.1088/0268-1242/26/6/064006 ↗
20. 10.1063/1.504529910.1063/1.5045299 ↗
21. 10.1063/1.349121510.1063/1.3491215 ↗
22. 10.1038/nature0148410.1038/nature01484 ↗
23. 10.1109/TASC.2007.89740310.1109/TASC.2007.897403 ↗
24. 10.1063/1.497682310.1063/1.4976823 ↗
25. 10.1016/j.diamond.2023.11034810.1016/j.diamond.2023.110348 ↗
26. 10.1103/PhysRevX.5.04100110.1103/PhysRevX.5.041001 ↗
27. 10.1103/PhysRevA.95.05341710.1103/PhysRevA.95.053417 ↗
28. 10.1063/5.006919510.1063/5.0069195 ↗
29. 10.1088/1751-8121/ab282810.1088/1751-8121/ab2828 ↗
30. De Pasquale, A.; Stace, T. M. Thermodynamics in the Quantum Regime: Fundamental Aspects and New Directions; Binder, F.; Correa, L. A.; Gogolin, C.; Anders, J.; Adesso, G., Eds. Springer International Publishing: Cham, 2018; pp 503–527.
31. 10.1088/1361-6528/ac1fb110.1088/1361-6528/ac1fb1 ↗
32. 10.1021/nl401216y10.1021/nl401216y ↗
33. 10.1063/1.131034510.1063/1.1310345 ↗
34. 10.1103/PhysRevX.2.03100110.1103/PhysRevX.2.031001 ↗
35. 10.1063/1.115071510.1063/1.1150715 ↗
36. 10.1063/1.138726210.1063/1.1387262 ↗
37. 10.1126/science.281.5379.94510.1126/science.281.5379.945 ↗
38. 10.1016/j.cossms.2024.10114810.1016/j.cossms.2024.101148 ↗
39. 10.1103/PhysRevB.85.20520310.1103/PhysRevB.85.205203 ↗
40. 10.1038/s41467-021-24725-110.1038/s41467-021-24725-1 ↗
41. 10.1038/nphys107510.1038/nphys1075 ↗
42. 10.1103/PhysRevB.84.19520410.1103/PhysRevB.84.195204 ↗
43. 10.1103/PhysRevB.101.06410210.1103/PhysRevB.101.064102 ↗
44. 10.1103/PhysRevB.106.05411010.1103/PhysRevB.106.054110 ↗
45. 10.1103/PhysRev.80.58010.1103/PhysRev.80.580 ↗
46. 10.1103/PhysRev.137.A6110.1103/PhysRev.137.A61 ↗
47. 10.1126/science.113187110.1126/science.1131871 ↗
48. 10.1103/PhysRevA.58.273310.1103/PhysRevA.58.2733 ↗
49. 10.1038/s41467-017-01159-210.1038/s41467-017-01159-2 ↗
50. 10.1021/acs.nanolett.0c0033910.1021/acs.nanolett.0c00339 ↗
51. Levitt M. H. · 2008
52. 10.1103/PhysRevLett.112.08760110.1103/PhysRevLett.112.087601 ↗
53. 10.1103/PhysRevApplied.10.05401010.1103/PhysRevApplied.10.054010 ↗
54. 10.1103/PhysRevB.100.09410410.1103/PhysRevB.100.094104 ↗
55. 10.1038/s41567-019-0420-010.1038/s41567-019-0420-0 ↗
56. 10.1103/PhysRevLett.125.10770210.1103/PhysRevLett.125.107702 ↗
57. 10.1103/PhysRevB.95.08140510.1103/PhysRevB.95.081405 ↗
58. 10.1038/s41928-023-01029-410.1038/s41928-023-01029-4 ↗
59. 10.1103/PhysRevLett.114.13640210.1103/PhysRevLett.114.136402 ↗
60. 10.1038/s41467-017-01993-410.1038/s41467-017-01993-4 ↗
61. 10.1073/pnas.180699811510.1073/pnas.1806998115 ↗
62. 10.1103/PhysRevLett.122.07610110.1103/PhysRevLett.122.076101 ↗
63. 10.1021/acsnano.8b0126510.1021/acsnano.8b01265 ↗
64. 10.1103/PhysRevApplied.11.06400310.1103/PhysRevApplied.11.064003 ↗
65. 10.1038/ncomms957710.1038/ncomms9577 ↗
66. 10.1126/science.aav278910.1126/science.aav2789 ↗
67. 10.1063/5.007966710.1063/5.0079667 ↗
68. 10.1103/PhysRevB.95.04140210.1103/PhysRevB.95.041402 ↗
69. 10.1038/s41467-021-24494-x10.1038/s41467-021-24494-x ↗
70. 10.1038/s41598-020-57569-810.1038/s41598-020-57569-8 ↗
71. 10.1038/s41467-019-13545-z10.1038/s41467-019-13545-z ↗
72. 10.1063/5.011592810.1063/5.0115928 ↗
73. 10.1103/PhysRevApplied.8.04401510.1103/PhysRevApplied.8.044015 ↗
74. 10.1063/1.490281810.1063/1.4902818 ↗
75. 10.1364/OPTICA.39862810.1364/OPTICA.398628 ↗
76. 10.1038/nphoton.2015.10310.1038/nphoton.2015.103 ↗
77. 10.1007/s11468-016-0384-110.1007/s11468-016-0384-1 ↗
78. 10.1038/s41598-017-14227-w10.1038/s41598-017-14227-w ↗
79. 10.1021/acs.nanolett.1c0249510.1021/acs.nanolett.1c02495 ↗
80. 10.1038/ncomms277110.1038/ncomms2771 ↗
81. 10.3390/ma1218295110.3390/ma12182951 ↗
82. 10.1038/s41467-021-22239-410.1038/s41467-021-22239-4 ↗
83. 10.1038/s41534-022-00622-310.1038/s41534-022-00622-3 ↗
84. 10.1038/s41563-023-01645-710.1038/s41563-023-01645-7 ↗
85. 10.1146/annurev-physchem-040513-10365910.1146/annurev-physchem-040513-103659 ↗
86. 10.1088/0034-4885/77/5/05650310.1088/0034-4885/77/5/056503 ↗
87. 10.1038/nphys196910.1038/nphys1969 ↗
88. 10.1103/PhysRevLett.104.07080110.1103/PhysRevLett.104.070801 ↗
89. 10.1038/natrevmats.2017.8810.1038/natrevmats.2017.88 ↗
90. 10.1038/nature1207210.1038/nature12072 ↗
91. 10.3390/diagnostics1205116410.3390/diagnostics12051164 ↗
92. 10.1073/pnas.160151311310.1073/pnas.1601513113 ↗
93. 10.1038/ncomms327910.1038/ncomms3279 ↗
94. 10.1126/science.125011310.1126/science.1250113 ↗
95. 10.1021/acsnano.3c1063310.1021/acsnano.3c10633 ↗
96. 10.1038/s41928-019-0275-510.1038/s41928-019-0275-5 ↗
97. 10.1021/nl501841d10.1021/nl501841d ↗
98. 10.1021/acsnanoscienceau.3c0005110.1021/acsnanoscienceau.3c00051 ↗
99. 10.1021/acsami.0c0154510.1021/acsami.0c01545 ↗
100. 10.1038/nature1237310.1038/nature12373 ↗