journal article·2024-01-30

Giant Ultrafast All-Optical Modulation Based on Exceptional Points in Exciton–Polariton Perovskite Metasurfaces

Mikhail A. Masharin, Tatiana Oskolkova, Furkan Isik, Hilmi Volkan Demir, Anton K. Samusev, Sergey V. Makarov

ACS Nano· Volume 18· Issue 4
Publisher page

Abstract

Ultrafast all-optical modulation with optically resonant nanostructures is an essential technology for high-speed signal processing on a compact optical chip. Key challenges that exist in this field are relatively low and slow modulations in the visible range as well as the use of expensive materials. Here we develop an ultrafast all-optical modulator based on MAPbBr 3 perovskite metasurface supporting exciton–polariton states with exceptional points. The additional angular and spectral filtering of the modulated light transmitted through the designed metasurface allows us to achieve 2500% optical signal modulation with the shortest modulation time of 440 fs at the pump fluence of ∼40 μJ/cm 2 . Such a value of the modulation depth is record-high among the existing modulators in the visible range, while the main physical effect behind it is polariton condensation. Scalable and cheap metasurface fabrication via nanoimprint lithography along with the simplicity of perovskite synthesis and deposition make the developed approach promising for real-life applications.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Strong Light-Matter Interactions · Perovskite Materials and Applications · Nonlinear Photonic Systems

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

UNAM-Institute of Materials Science and Nanotechnology, National Nanotechnology Research Center, Department of Electrical and Electronics Engineering, Department of Physics, Bilkent University, Ankara 06800, Turkey

Laboratory of Bionanophotonic, Institute of Bioengineering, École Polytechnique Fédérale de Lausanne (EPFL), Lausanne 1015, Switzerland

LUMINOUS! Center of Excellence for Semiconductor Lighting and Displays, School of Electrical and Electronic Engineering, School of Physical and Mathematical Sciences, School of Materials Science and Engineering, Nanyang Technological University, 639798, Singapore

Experimentelle Physik 2, Technische Universität Dortmund, Dortmund 44227, Germany

Qingdao Innovation and Development Center, Harbin Engineering University, Qingdao, Shandong 266000, China

Funding

Deutsche Forschungsgemeinschaft · Excellent Young Scientists Fund

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