journal article·2016-07-26Open access

High-Efficiency Light-Emitting Diodes of Organometal Halide Perovskite Amorphous Nanoparticles

Jun Xing, Fei Yan, Yawen Zhao, Shi Chen, Huakang Yu, Qing Zhang, Rongguang Zeng, Hilmi Volkan Demir, Xiaowei Sun, Alfred Huan, Qihua Xiong

ACS Nano· Volume 10· Issue 7

Abstract

Organometal halide perovskite has recently emerged as a very promising family of materials with augmented performance in electronic and optoelectronic applications including photovoltaic devices, photodetectors, and light-emitting diodes. Herein, we propose and demonstrate facile solution synthesis of a series of colloidal organometal halide perovskite CH3NH3PbX3 (X = halides) nanoparticles with amorphous structure, which exhibit high quantum yield and tunable emission from ultraviolet to near-infrared. The growth mechanism and photoluminescence properties of the perovskite amorphous nanoparticles were studied in detail. A high-efficiency green-light-emitting diode based on amorphous CH3NH3PbBr3 nanoparticles was demonstrated. The perovskite amorphous nanoparticle-based light-emitting diode shows a maximum luminous efficiency of 11.49 cd/A, a power efficiency of 7.84 lm/W, and an external quantum efficiency of 3.8%, which is 3.5 times higher than that of the best colloidal perovskite quantum-dot-based light-emitting diodes previously reported. Our findings indicate the great potential of colloidal perovskite amorphous nanoparticles in light-emitting devices.
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Research context

OpenAlex topics: Perovskite Materials and Applications · Organic Light-Emitting Diodes Research · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore 637371

LUMINOUS! Center of Excellence for Semiconductor Lighting and Displays, TPI-The Photonics Institute, School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore 639798

China Academy of Engineering Physics, Mianyang 621900, China

Department of Electrical and Electronics Engineering, Department of Physics, UNAM−Institute of Materials Science and Nanotechnology, Bilkent University, Ankara 06800, Turkey

NOVITAS, Nanoelectronics Centre of Excellence, School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore 639798

Funding

Agency for Science, Technology and Research · Ministry of Education - Singapore · National Research Foundation-Prime Minister's office, Republic of Singapore · T?rkiye Bilimler Akademisi

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