journal article·2024-01-12Open access

Scale-up Solutions of 2D Perovskite Photovoltaics: Insights of Multiscale Structures

Junke Jiang, Jiaxue You, Shengzhong Frank Liu, Jun Xi

ACS Energy Letters· Volume 9· Issue 1

Abstract

Two-dimensional (2D) perovskites assembled with hydrophobic bulky organic cations demonstrate much enhanced ambient stability and anisotropic carrier transport, making their devices highly promising. However, photovoltaic (PV) devices scaling up to modules using 2D perovskites lag far behind their 3D counterparts. Hence, improving the scalability and efficiency of 2D perovskite PV devices is a challenging topic. In this Perspective, from the insights of multiscale structures of 2D perovskites, we analyze the interrelated causes and propose rational solutions to these two issues. The scalability issue is scrutinized from the structures of the born inks and the ended films. The efficiency issue is investigated from the structures of the phase landscape and the lattice anharmonicity. Finally, the collective and fine moiety effect for material structure, the state-of-the-art computational methodologies, as well as the machine-learning-based diagnosis are discussed. We hope this Perspective can accelerate the roadmap for building 2D perovskite PV fab.
Source: openalex_inverted_index · Quality: baseline

Research context

OpenAlex topics: Perovskite Materials and Applications · 2D Materials and Applications · Quantum Dots Synthesis And Properties

SciVX discovery tags are terminology-based. OpenAlex topics are source-provided classifications.

Affiliations

Materials Simulation & Modelling, Department of Applied Physics, Eindhoven University of Technology and Center for Computational Energy Research, Department of Applied Physics, Eindhoven University of Technology, 5600 MB Eindhoven, The Netherlands

Department of Materials Science and Engineering, Hong Kong Institute for Clean Energy, City University of Hong Kong, Hong Kong SAR, China

Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science & Engineering, Shaanxi Normal University, Xi’an 710119, China

Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi Key Lab of Information Photonic Technique, School of Electronic Science and Engineering, Xi’an Jiaotong University, No. 28, Xianning West Road, Xi’an 710049, China

Funding

Dalian National Laboratory for Clean Energy · National Key Research and Development Program of China · Yulin University · National Natural Science Foundation of China · Xi'an Jiaotong University Young Talents Support Program · Xi'an Jiaotong University

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